001     607366
005     20240611213405.0
024 7 _ |a arXiv:1910.13494
|2 arXiv
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024 7 _ |a pmid:32113333
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037 _ _ |a PUBDB-2024-01855
041 _ _ |a English
082 _ _ |a 530
088 _ _ |a arXiv:1910.13494
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100 1 _ |a Kierspel, Thomas
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245 _ _ |a X-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame
260 _ _ |c 2020
336 7 _ |a Preprint
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336 7 _ |a WORKING_PAPER
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336 7 _ |a Electronic Article
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336 7 _ |a preprint
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336 7 _ |a ARTICLE
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520 _ _ |a We report experimental results on the diffractive imaging of three-dimensionally aligned 2,5-diiodothiophene molecules. The molecules were aligned by chirped near-infrared laser pulses, and their structure was probed at a photon energy of 9.5 keV ($\lambda\approx130 \text{pm}$) provided by the Linac Coherent Light Source. Diffracted photons were recorded on the CSPAD detector and a two-dimensional diffraction pattern of the equilibrium structure of 2,5-diiodothiophene was recorded. The retrieved distance between the two iodine atoms agrees with the quantum-chemically calculated molecular structure to within 5 %. The experimental approach allows for the imaging of intrinsic molecular dynamics in the molecular frame, albeit this requires more experimental data which should be readily available at upcoming high-repetition-rate facilities.
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536 _ _ |a Ex-Net-0002-Phase2-3 - Advanced Imaging of Matter: Structure, Dynamics and Control on the Atomic Scale - AIM (2018_Ex-Net-0002-Phase2-3)
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536 _ _ |a MEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789)
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536 _ _ |a DFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)
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536 _ _ |a DFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)
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700 1 _ |a Christensen, Lauge
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700 1 _ |a Fry, Alan
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700 1 _ |a Hunter, Mark
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700 1 _ |a Koglin, Jason E.
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700 1 _ |a Liang, Mengning
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700 1 _ |a Mariani, Valerio
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700 1 _ |a Natan, Adi
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700 1 _ |a Robinson, Joseph
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700 1 _ |a Rolles, Daniel
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700 1 _ |a Rudenko, Artem
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700 1 _ |a Schnorr, Kirsten
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700 1 _ |a Stapelfeldt, Henrik
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700 1 _ |a Stern, Stephan
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700 1 _ |a Thøgersen, Jan
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700 1 _ |a Yoon, Chun Hong
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700 1 _ |a Wang, Fenglin
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700 1 _ |a Küpper, Jochen
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