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@ARTICLE{Kierspel:607366,
author = {Kierspel, Thomas and Morgan, Andrew and Wiese, Joss and
Mullins, Terry and Aquila, Andy and Barty, Anton and Bean,
Richard and Boll, Rebecca and Boutet, Sébastien and
Bucksbaum, Philip and Chapman, Henry N. and Christensen,
Lauge and Fry, Alan and Hunter, Mark and Koglin, Jason E.
and Liang, Mengning and Mariani, Valerio and Natan, Adi and
Robinson, Joseph and Rolles, Daniel and Rudenko, Artem and
Schnorr, Kirsten and Stapelfeldt, Henrik and Stern, Stephan
and Thøgersen, Jan and Yoon, Chun Hong and Wang, Fenglin
and Küpper, Jochen},
title = {{X}-ray diffractive imaging of controlled gas-phase
molecules: {T}oward imaging of dynamics in the molecular
frame},
reportid = {PUBDB-2024-01855, arXiv:1910.13494},
year = {2020},
abstract = {We report experimental results on the diffractive imaging
of three-dimensionally aligned 2,5-diiodothiophene
molecules. The molecules were aligned by chirped
near-infrared laser pulses, and their structure was probed
at a photon energy of 9.5 keV ($\lambda\approx130
\text{pm}$) provided by the Linac Coherent Light Source.
Diffracted photons were recorded on the CSPAD detector and a
two-dimensional diffraction pattern of the equilibrium
structure of 2,5-diiodothiophene was recorded. The retrieved
distance between the two iodine atoms agrees with the
quantum-chemically calculated molecular structure to within
5 \%. The experimental approach allows for the imaging of
intrinsic molecular dynamics in the molecular frame, albeit
this requires more experimental data which should be readily
available at upcoming high-repetition-rate facilities.},
cin = {FS-CFEL-CMI / UNI/CUI / UNI/EXP / FS-CFEL-1},
ddc = {530},
cid = {I:(DE-H253)FS-CFEL-CMI-20220405 /
$I:(DE-H253)UNI_CUI-20121230$ /
$I:(DE-H253)UNI_EXP-20120731$ /
I:(DE-H253)FS-CFEL-1-20120731},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / Ex-Net-0002-Phase2-3 - Advanced Imaging of
Matter: Structure, Dynamics and Control on the Atomic Scale
- AIM $(2018_Ex-Net-0002-Phase2-3)$ / VH-VI-419 - Dynamic
Pathways in Multidimensional Landscapes (VH-VI-419) /
COMOTION - Controlling the Motion of Complex Molecules and
Particles (614507) / MEDEA - Molecular Electron Dynamics
investigated by IntensE Fields and Attosecond Pulses
(641789) / DFG project 390715994 - EXC 2056: CUI: Advanced
Imaging of Matter (390715994) / DFG project 194651731 - EXC
1074: Hamburger Zentrum für ultraschnelle Beobachtung
(CUI): Struktur, Dynamik und Kontrolle von Materie auf
atomarer Skala (194651731)},
pid = {G:(DE-HGF)POF4-631 / $G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$
/ G:(DE-HGF)VH-VI-419 / G:(EU-Grant)614507 /
G:(EU-Grant)641789 / G:(GEPRIS)390715994 /
G:(GEPRIS)194651731},
experiment = {EXP:(DE-H253)CFEL-Exp-20150101},
typ = {PUB:(DE-HGF)25},
eprint = {1910.13494},
howpublished = {arXiv:1910.13494},
archivePrefix = {arXiv},
SLACcitation = {$\%\%CITATION$ = $arXiv:1910.13494;\%\%$},
pubmed = {pmid:32113333},
url = {https://bib-pubdb1.desy.de/record/607366},
}