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000607366 005__ 20240611213405.0
000607366 0247_ $$2arXiv$$aarXiv:1910.13494
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000607366 088__ $$2arXiv$$aarXiv:1910.13494
000607366 1001_ $$0P:(DE-H253)PIP1018289$$aKierspel, Thomas$$b0$$udesy
000607366 245__ $$aX-ray diffractive imaging of controlled gas-phase molecules: Toward imaging of dynamics in the molecular frame
000607366 260__ $$c2020
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000607366 520__ $$aWe report experimental results on the diffractive imaging of three-dimensionally aligned 2,5-diiodothiophene molecules. The molecules were aligned by chirped near-infrared laser pulses, and their structure was probed at a photon energy of 9.5 keV ($\lambda\approx130 \text{pm}$) provided by the Linac Coherent Light Source. Diffracted photons were recorded on the CSPAD detector and a two-dimensional diffraction pattern of the equilibrium structure of 2,5-diiodothiophene was recorded. The retrieved distance between the two iodine atoms agrees with the quantum-chemically calculated molecular structure to within 5 %. The experimental approach allows for the imaging of intrinsic molecular dynamics in the molecular frame, albeit this requires more experimental data which should be readily available at upcoming high-repetition-rate facilities.
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000607366 536__ $$0G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$$aEx-Net-0002-Phase2-3 - Advanced Imaging of Matter: Structure, Dynamics and Control on the Atomic Scale - AIM (2018_Ex-Net-0002-Phase2-3)$$c2018_Ex-Net-0002-Phase2-3$$x1
000607366 536__ $$0G:(DE-HGF)VH-VI-419$$aVH-VI-419 - Dynamic Pathways in Multidimensional Landscapes (VH-VI-419)$$cVH-VI-419$$x2
000607366 536__ $$0G:(EU-Grant)614507$$aCOMOTION - Controlling the Motion of Complex Molecules and Particles (614507)$$c614507$$fERC-2013-CoG$$x3
000607366 536__ $$0G:(EU-Grant)641789$$aMEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789)$$c641789$$fH2020-MSCA-ITN-2014$$x4
000607366 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x5
000607366 536__ $$0G:(GEPRIS)194651731$$aDFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)$$c194651731$$x6
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000607366 7001_ $$0P:(DE-H253)PIP1014904$$aMorgan, Andrew$$b1
000607366 7001_ $$0P:(DE-H253)PIP1022847$$aWiese, Joss$$b2
000607366 7001_ $$0P:(DE-HGF)0$$aMullins, Terry$$b3
000607366 7001_ $$0P:(DE-HGF)0$$aAquila, Andy$$b4
000607366 7001_ $$0P:(DE-H253)PIP1008245$$aBarty, Anton$$b5$$udesy
000607366 7001_ $$0P:(DE-H253)PIP1016993$$aBean, Richard$$b6
000607366 7001_ $$0P:(DE-H253)PIP1014282$$aBoll, Rebecca$$b7
000607366 7001_ $$0P:(DE-H253)PIP1009086$$aBoutet, Sébastien$$b8
000607366 7001_ $$0P:(DE-H253)PIP1009467$$aBucksbaum, Philip$$b9
000607366 7001_ $$0P:(DE-H253)PIP1006324$$aChapman, Henry N.$$b10
000607366 7001_ $$0P:(DE-H253)PIP1013267$$aChristensen, Lauge$$b11
000607366 7001_ $$00000-0002-3339-3176$$aFry, Alan$$b12
000607366 7001_ $$0P:(DE-H253)PIP1009944$$aHunter, Mark$$b13
000607366 7001_ $$0P:(DE-HGF)0$$aKoglin, Jason E.$$b14
000607366 7001_ $$0P:(DE-H253)PIP1007507$$aLiang, Mengning$$b15
000607366 7001_ $$0P:(DE-H253)PIP1021498$$aMariani, Valerio$$b16$$udesy
000607366 7001_ $$0P:(DE-H253)PIP1090478$$aNatan, Adi$$b17
000607366 7001_ $$0P:(DE-HGF)0$$aRobinson, Joseph$$b18
000607366 7001_ $$0P:(DE-H253)PIP1007320$$aRolles, Daniel$$b19
000607366 7001_ $$0P:(DE-H253)PIP1006803$$aRudenko, Artem$$b20
000607366 7001_ $$0P:(DE-H253)PIP1013918$$aSchnorr, Kirsten$$b21
000607366 7001_ $$aStapelfeldt, Henrik$$b22
000607366 7001_ $$aStern, Stephan$$b23
000607366 7001_ $$0P:(DE-HGF)0$$aThøgersen, Jan$$b24
000607366 7001_ $$0P:(DE-H253)PIP1016300$$aYoon, Chun Hong$$b25
000607366 7001_ $$0P:(DE-H253)PIP1006747$$aWang, Fenglin$$b26
000607366 7001_ $$0P:(DE-H253)PIP1012175$$aKüpper, Jochen$$b27$$eCorresponding author
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