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| Home > Publications database > Laser-induced Coulomb explosion imaging of $(C_6$$H_5$$Br)$$_2$ and $C_6$$H_5$$Br$-$I_2$ dimers in helium nanodroplets using the Timepix3 > print |
| Home > Publications database > Laser-induced Coulomb explosion imaging of $(C_6$$H_5$$Br)$$_2$ and $C_6$$H_5$$Br$-$I_2$ dimers in helium nanodroplets using the Timepix3 > print |
| 001 | 607361 | ||
| 005 | 20240602054159.0 | ||
| 024 | 7 | _ | |a arXiv:2105.00764 |2 arXiv |
| 024 | 7 | _ | |a 10.3204/PUBDB-2024-01850 |2 datacite_doi |
| 037 | _ | _ | |a PUBDB-2024-01850 |
| 041 | _ | _ | |a English |
| 082 | _ | _ | |a 530 |
| 088 | _ | _ | |a arXiv:2105.00764 |2 arXiv |
| 100 | 1 | _ | |a Schouder, Constant |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Laser-induced Coulomb explosion imaging of $(C_6$$H_5$$Br)$$_2$ and $C_6$$H_5$$Br$-$I_2$ dimers in helium nanodroplets using the Timepix3 |
| 260 | _ | _ | |c 2021 |
| 336 | 7 | _ | |a Preprint |b preprint |m preprint |0 PUB:(DE-HGF)25 |s 1716813040_2811274 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a WORKING_PAPER |2 ORCID |
| 336 | 7 | _ | |a Electronic Article |0 28 |2 EndNote |
| 336 | 7 | _ | |a preprint |2 DRIVER |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a Output Types/Working Paper |2 DataCite |
| 520 | _ | _ | |a We have deduced the structure of the bromobenzene-$I_2$ heterodimer and the bromobenzene homodimer inside helium droplets using a combination of laser-induced alignment, Coulomb explosion imaging, and three-dimensional ion imaging. The complexes were fixed in a variety of orientations in the laboratory frame, then in each case multiply ionized by an intense laser pulse. A three dimensional ion imaging detector, including a Timepix3 detector allowed us to measure the correlations between velocity vectors of different fragments and, in conjunction with classical simulations, work backward to the initial structure of the complex prior to explosion. For the heterodimer, we find that the $I_2$ molecular axis intersects the phenyl ring of the bromobenzene approximately perpendicularly. The homodimer has a stacked parallel structure, with the two bromine atoms pointing in opposite directions. These results illustrate the ability of Coulomb explosion imaging to determine the structure of large complexes, and point the way toward real-time measurements of bimolecular reactions inside helium droplets. |
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| 536 | _ | _ | |a MEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789) |0 G:(EU-Grant)641789 |c 641789 |f H2020-MSCA-ITN-2014 |x 1 |
| 536 | _ | _ | |a ASPIRE - Angular studies of photoelectrons in innovative research environments (674960) |0 G:(EU-Grant)674960 |c 674960 |f H2020-MSCA-ITN-2015 |x 2 |
| 536 | _ | _ | |a DFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994) |0 G:(GEPRIS)390715994 |c 390715994 |x 3 |
| 536 | _ | _ | |a Ex-Net-0002-Phase2-3 - Advanced Imaging of Matter: Structure, Dynamics and Control on the Atomic Scale - AIM (2018_Ex-Net-0002-Phase2-3) |0 G:(DE-HGF)2018_Ex-Net-0002-Phase2-3 |c 2018_Ex-Net-0002-Phase2-3 |x 4 |
| 588 | _ | _ | |a Dataset connected to arXivarXiv, CrossRef, Journals: bib-pubdb1.desy.de |
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| 700 | 1 | _ | |a Chatterley, Adam S |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Johny, Melby |0 P:(DE-H253)PIP1028301 |b 2 |
| 700 | 1 | _ | |a Hübschmann, Flora |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Al-Refaie, Ahmed F |0 P:(DE-H253)PIP1081972 |b 4 |
| 700 | 1 | _ | |a Calvo, Florent |0 0000-0002-3621-3046 |b 5 |
| 700 | 1 | _ | |a Küpper, Jochen |0 P:(DE-H253)PIP1012175 |b 6 |
| 700 | 1 | _ | |a Stapelfeldt, Henrik |0 P:(DE-H253)PIP1085121 |b 7 |e Corresponding author |
| 856 | 4 | _ | |y OpenAccess |u https://bib-pubdb1.desy.de/record/607361/files/arxiv%20pdf.pdf |
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