000607361 001__ 607361
000607361 005__ 20240602054159.0
000607361 0247_ $$2arXiv$$aarXiv:2105.00764
000607361 0247_ $$2datacite_doi$$a10.3204/PUBDB-2024-01850
000607361 037__ $$aPUBDB-2024-01850
000607361 041__ $$aEnglish
000607361 082__ $$a530
000607361 088__ $$2arXiv$$aarXiv:2105.00764
000607361 1001_ $$0P:(DE-HGF)0$$aSchouder, Constant$$b0
000607361 245__ $$aLaser-induced Coulomb explosion imaging of $(C_6$$H_5$$Br)$$_2$ and $C_6$$H_5$$Br$-$I_2$ dimers in helium nanodroplets using the Timepix3 
000607361 260__ $$c2021
000607361 3367_ $$0PUB:(DE-HGF)25$$2PUB:(DE-HGF)$$aPreprint$$bpreprint$$mpreprint$$s1716813040_2811274
000607361 3367_ $$2ORCID$$aWORKING_PAPER
000607361 3367_ $$028$$2EndNote$$aElectronic Article
000607361 3367_ $$2DRIVER$$apreprint
000607361 3367_ $$2BibTeX$$aARTICLE
000607361 3367_ $$2DataCite$$aOutput Types/Working Paper
000607361 520__ $$aWe have deduced the structure of the bromobenzene-$I_2$ heterodimer and the bromobenzene homodimer inside helium droplets using a combination of laser-induced alignment, Coulomb explosion imaging, and three-dimensional ion imaging. The complexes were fixed in a variety of orientations in the laboratory frame, then in each case multiply ionized by an intense laser pulse. A three dimensional ion imaging detector, including a Timepix3 detector allowed us to measure the correlations between velocity vectors of different fragments and, in conjunction with classical simulations, work backward to the initial structure of the complex prior to explosion. For the heterodimer, we find that the $I_2$ molecular axis intersects the phenyl ring of the bromobenzene approximately perpendicularly. The homodimer has a stacked parallel structure, with the two bromine atoms pointing in opposite directions. These results illustrate the ability of Coulomb explosion imaging to determine the structure of large complexes, and point the way toward real-time measurements of bimolecular reactions inside helium droplets. 
000607361 536__ $$0G:(DE-HGF)POF4-631$$a631 - Matter – Dynamics, Mechanisms and Control (POF4-631)$$cPOF4-631$$fPOF IV$$x0
000607361 536__ $$0G:(EU-Grant)641789$$aMEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789)$$c641789$$fH2020-MSCA-ITN-2014$$x1
000607361 536__ $$0G:(EU-Grant)674960$$aASPIRE - Angular studies of photoelectrons in innovative research environments (674960)$$c674960$$fH2020-MSCA-ITN-2015$$x2
000607361 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x3
000607361 536__ $$0G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$$aEx-Net-0002-Phase2-3 - Advanced Imaging of Matter: Structure, Dynamics and Control on the Atomic Scale - AIM (2018_Ex-Net-0002-Phase2-3)$$c2018_Ex-Net-0002-Phase2-3$$x4
000607361 588__ $$aDataset connected to arXivarXiv, CrossRef, Journals: bib-pubdb1.desy.de
000607361 693__ $$0EXP:(DE-H253)CFEL-Exp-20150101$$5EXP:(DE-H253)CFEL-Exp-20150101$$eExperiments at CFEL$$x0
000607361 7001_ $$0P:(DE-HGF)0$$aChatterley, Adam S$$b1
000607361 7001_ $$0P:(DE-H253)PIP1028301$$aJohny, Melby$$b2
000607361 7001_ $$0P:(DE-HGF)0$$aHübschmann, Flora$$b3
000607361 7001_ $$0P:(DE-H253)PIP1081972$$aAl-Refaie, Ahmed F$$b4
000607361 7001_ $$00000-0002-3621-3046$$aCalvo, Florent$$b5
000607361 7001_ $$0P:(DE-H253)PIP1012175$$aKüpper, Jochen$$b6
000607361 7001_ $$0P:(DE-H253)PIP1085121$$aStapelfeldt, Henrik$$b7$$eCorresponding author
000607361 8564_ $$uhttps://bib-pubdb1.desy.de/record/607361/files/arxiv%20pdf.pdf$$yOpenAccess
000607361 8564_ $$uhttps://bib-pubdb1.desy.de/record/607361/files/arxiv%20pdf.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000607361 909CO $$ooai:bib-pubdb1.desy.de:607361$$pdnbdelivery$$pec_fundedresources$$pVDB$$pdriver$$popen_access$$popenaire
000607361 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1028301$$aCentre for Free-Electron Laser Science$$b2$$kCFEL
000607361 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1028301$$aExternal Institute$$b2$$kExtern
000607361 9101_ $$0I:(DE-588)1043621512$$6P:(DE-H253)PIP1028301$$aEuropean XFEL$$b2$$kXFEL.EU
000607361 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1081972$$aExternal Institute$$b4$$kExtern
000607361 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1012175$$aDeutsches Elektronen-Synchrotron$$b6$$kDESY
000607361 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1012175$$aCentre for Free-Electron Laser Science$$b6$$kCFEL
000607361 9101_ $$0I:(DE-588)1043621512$$6P:(DE-H253)PIP1012175$$aEuropean XFEL$$b6$$kXFEL.EU
000607361 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1085121$$aExternal Institute$$b7$$kExtern
000607361 9101_ $$0I:(DE-588)1043621512$$6P:(DE-H253)PIP1085121$$aEuropean XFEL$$b7$$kXFEL.EU
000607361 9131_ $$0G:(DE-HGF)POF4-631$$1G:(DE-HGF)POF4-630$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vMatter – Dynamics, Mechanisms and Control$$x0
000607361 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000607361 915__ $$0LIC:(DE-HGF)CCBY4$$2HGFVOC$$aCreative Commons Attribution CC BY 4.0
000607361 915__ $$0StatID:(DE-HGF)0580$$2StatID$$aPublished
000607361 9201_ $$0I:(DE-H253)FS-CFEL-CMI-20220405$$kFS-CFEL-CMI$$lCFEL-CMI$$x0
000607361 9201_ $$0I:(DE-H253)UNI_CUI-20121230$$kUNI/CUI$$lbeauftragt von UNI$$x1
000607361 9201_ $$0I:(DE-H253)UNI_EXP-20120731$$kUNI/EXP$$lUni Hamburg / Experimentalphysik$$x2
000607361 980__ $$apreprint
000607361 980__ $$aVDB
000607361 980__ $$aUNRESTRICTED
000607361 980__ $$aI:(DE-H253)FS-CFEL-CMI-20220405
000607361 980__ $$aI:(DE-H253)UNI_CUI-20121230
000607361 980__ $$aI:(DE-H253)UNI_EXP-20120731
000607361 9801_ $$aFullTexts