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@ARTICLE{Podoliak:607037,
author = {Podoliak, E. and Lamm, G. H. U. and Marin, E. and
Schellbach, A. V. and Fedotov, D. A. and Stetsenko, A. and
Asido, M. and Maliar, N. and Bourenkov, G. and Balandin, T.
and Baeken, C. and Astashkin, R. and Schneider, T. R. and
Bateman, A. and Wachtveitl, J. and Schapiro, I. and
Busskamp, V. and Guskov, A. and Gordeliy, V. and Alekseev,
A. and Kovalev, K.},
title = {{A} subgroup of light-driven sodium pumps with an
additional {S}chiff base counterion},
journal = {Nature Communications},
volume = {15},
number = {1},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {PUBDB-2024-01742},
pages = {3119},
year = {2024},
abstract = {Light-driven sodium pumps (NaRs) are unique
ion-transporting microbial rhodopsins. The major group of
NaRs is characterized by an NDQ motif and has two aspartic
acid residues in the central region essential for sodium
transport. Here we identify a subgroup of the NDQ rhodopsins
bearing an additional glutamic acid residue in the close
vicinity to the retinal Schiff base. We thoroughly
characterize a member of this subgroup, namely the protein
ErNaR from Erythrobacter sp. HL-111 and show that the
additional glutamic acid results in almost complete loss of
pH sensitivity for sodium-pumping activity, which is in
contrast to previously studied NaRs. ErNaR is capable of
transporting sodium efficiently even at acidic pH levels.
X-ray crystallography and single particle cryo-electron
microscopy reveal that the additional glutamic acid residue
mediates the connection between the other two Schiff base
counterions and strongly interacts with the aspartic acid of
the characteristic NDQ motif. Hence, it reduces its pKa. Our
findings shed light on a subgroup of NaRs and might serve as
a basis for their rational optimization for optogenetics.},
cin = {EMBL-User / EMBL},
ddc = {500},
cid = {I:(DE-H253)EMBL-User-20120814 / I:(DE-H253)EMBL-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / DFG project
G:(GEPRIS)390729940 - EXC 2067: Multiscale Bioimaging: Von
molekularen Maschinen zu Netzwerken erregbarer Zellen
(390729940) / DFG project G:(GEPRIS)390873048 - EXC 2151:
ImmunoSensation2 - the immune sensory system (390873048)},
pid = {G:(DE-HGF)POF4-6G3 / G:(GEPRIS)390729940 /
G:(GEPRIS)390873048},
experiment = {EXP:(DE-H253)P-P14-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:38600129},
UT = {WOS:001202408400026},
doi = {10.1038/s41467-024-47469-0},
url = {https://bib-pubdb1.desy.de/record/607037},
}