TY - JOUR
AU - Shokeen, Vishal
AU - Heber, Michael
AU - Kutnyakhov, Dmytro
AU - Wang, Xiaocui
AU - Yaroslavtsev, Alexander
AU - Maldonado, Pablo
AU - Berritta, Marco
AU - Wind, Nils
AU - Wenthaus, Lukas
AU - Pressacco, Federico
AU - Min, Chul-Hee
AU - Nissen, Matz
AU - Mahatha, Sanjoy K.
AU - Dziarzhytski, Siarhei
AU - Oppeneer, Peter M.
AU - Rossnagel, Kai
AU - Elmers, Hans-Joachim
AU - Schoenhense, Gerd
AU - Duerr, Hermann
TI - Real-time observation of non-equilibrium phonon-electron energy and angular momentum flow in laser-heated nickel
JO - Science advances
VL - 10
IS - 5
SN - 2375-2548
CY - Washington, DC [u.a.]
PB - Assoc.
M1 - PUBDB-2024-01687
SP - eadj2407
PY - 2024
AB - Identifying the microscopic nature of non-equilibrium energy transfer mechanisms among electronic, spin, and lattice degrees of freedom is central to understanding ultrafast phenomena such as manipulating magnetism on the femtosecond timescale. Here, we use time- and angle-resolved photoemission spectroscopy to go beyond the often-used ensemble-averaged view of non-equilibrium dynamics in terms of quasiparticle temperature evolutions. We show for ferromagnetic Ni that the non-equilibrium electron and spin dynamics display pronounced variations with electron momentum, whereas the magnetic exchange interaction remains isotropic. This highlights the influence of lattice-mediated scattering processes and opens a pathway toward unraveling the still elusive microscopic mechanism of spin-lattice angular momentum transfer.
LB - PUB:(DE-HGF)16
C6 - pmid:38295169
UR - <Go to ISI:>//WOS:001185617600008
DO - DOI:10.1126/sciadv.adj2407
UR - https://bib-pubdb1.desy.de/record/606911
ER -