Preprint PUBDB-2024-01673

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Controlled molecule injector for cold, dense, and pure molecular beams at the European x-ray free-electron laser

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2024

 GO

Report No.: arXiv:2405.06344

Abstract: A permanently available molecular-beam injection setup for controlled molecules (COMO) was installed and commissioned at the small quantum systems (SQS) instrument at the European x-ray free-electron laser (EuXFEL). A $b$-type electrostatic deflector allows for pure state-, size-, and isomer-selected samples of polar molecules and clusters. The source provides a rotationally cold ($T\approx1$~K) and dense ($\rho\approx10^8$~cm$^{-3}$) molecular beam with pulse durations up to 100~\us generated by a new version of the Even-Lavie valve. Here, a performance overview of the COMO setup is presented along with characterization experiments performed both, with an optical laser at the Center for Free-Electron-Laser Science and with x-rays at EuXFEL under burst-mode operation. COMO was designed to be attached to different instruments at the EuXFEL, in particular at the small quantum systems (SQS) and single particles, clusters, and biomolecules (SPB) instruments. This advanced controlled-molecules injection setup enables XFEL studies using highly defined samples with soft and hard x-ray FEL radiation for applications ranging from atomic, molecular, and cluster physics to elementary processes in chemistry and biology.


Note: Prepring corresponding to https://bib-pubdb1.desy.de/record/586150

Contributing Institute(s):
  1. CFEL-CMI (FS-CFEL-CMI)
  2. The European XFEL Users (XFEL-User)
  3. beauftragt von UNI (UNI/CUI)
  4. Uni Hamburg / Experimentalphysik (UNI/EXP)
Research Program(s):
  1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
  2. MEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789) (641789)
  3. DFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994) (390715994)
  4. HIRS-0018 - Helmholtz-Lund International School - Intelligent instrumentation for exploring matter at different time and length scales (HELIOS) (2020_HIRS-0018) (2020_HIRS-0018)
  5. 05K22GUA - Verbundprojekt 05K2022 - 2021-05992 UDIET: Ultraschnelle Dynamik des intermolekularen Energietransfers: elementare Schritte in Aerosolen und Flüssigchemie (BMBF-05K22GUA) (BMBF-05K22GUA)
Experiment(s):
  1. Experiments at CFEL
  2. Experiments at XFEL

Appears in the scientific report 2024
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The record appears in these collections:
Private Collections > >Extern > >HAS-User > >FS-UNI > UNI/CUI
Private Collections > >Extern > >HAS-User > >FS-UNI > UNI/EXP
Private Collections > >DESY > >FS > FS-CFEL-CMI
Private Collections > >XFEL.EU > XFEL-User
Document types > Reports > Preprints
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Publications database

 Record created 2024-05-08, last modified 2024-08-29


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