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| 001 | 605553 | ||
| 005 | 20250723171711.0 | ||
| 024 | 7 | _ | |a 10.1002/adma.202313621 |2 doi |
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| 100 | 1 | _ | |a Du, Jingwei |0 P:(DE-H253)PIP1098080 |b 0 |
| 245 | _ | _ | |a A High‐Energy Tellurium Redox‐Amphoteric Conversion Cathode Chemistry for Aqueous Zinc Batteries |
| 260 | _ | _ | |a Weinheim |c 2024 |b Wiley-VCH |
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| 520 | _ | _ | |a Rechargeable aqueous zinc batteries are potential candidates for sustainable energy storage systems at a grid scale, owing to their high safety and low cost. However, the existing cathode chemistries exhibit restricted energy density, which hinders their extensive applications. Here, a tellurium redox-amphoteric conversion cathode chemistry is presented for aqueous zinc batteries, which delivers a specific capacity of 1223.9 mAh gTe$^{−1}$ and a high energy density of 1028.0 Wh kgTe$^{−1}$. A highly concentrated electrolyte (30 mol kg$^{−1}$ ZnCl$_2$) is revealed crucial for initiating the Te redox-amphoteric conversion as it suppresses the H$_2$O reactivity and inhibits undesirable hydrolysis of the Te$^{4+}$ product. By carrying out multiple operando/ex situ characterizations, the reversible six-electron Te$^{2−}$/Te$^0$/Te$^{4+}$ conversion with TeCl$_4$ is identified as the fully charged product and ZnTe as the fully discharged product. This finding not only enriches the conversion-type battery chemistries but also establishes a critical step in exploring redox-amphoteric materials for aqueous zinc batteries and beyond. |
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| 700 | 1 | _ | |a Zhao, Yirong |b 1 |
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| 700 | 1 | _ | |a Wang, Gang |0 P:(DE-H253)PIP1008694 |b 3 |
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| 700 | 1 | _ | |a Feng, Xinliang |0 P:(DE-H253)PIP1081776 |b 14 |e Corresponding author |
| 700 | 1 | _ | |a Yu, Minghao |0 P:(DE-H253)PIP1083931 |b 15 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/adma.202313621 |g p. 2313621 |0 PERI:(DE-600)1474949-X |n 19 |p 2313621 |t Advanced materials |v 36 |y 2024 |x 0935-9648 |
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