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@ARTICLE{Thesing:605154,
      author       = {Thesing, Linda and Yachmenev, Andrey and González-Férez,
                      Rosario and Küpper, Jochen},
      title        = {{M}olecular influence on nuclear-quadrupole coupling
                      effects in laser induced alignment},
      reportid     = {PUBDB-2024-01328, arXiv:2408.01125},
      year         = {2024},
      abstract     = {We studied the effect of nuclear-quadrupole interactions on
                      the field-free impulsive alignment of different
                      asymmetric-top molecules. Our analysis is focused on the
                      influence of the hyperfine- and rotational-energy-level
                      structures. These depend on the number of nuclear spins, the
                      rotational constants, and the symmetry of the tensors
                      involved in the nuclear spin and external field
                      interactions. Comparing the prototypical large-nuclear- spin
                      molecules iodobenzene, 1,2-diiodobenzene, 1,3-diiodobenzene,
                      and 2,5-diiodobenzonitrile, we demonstrate that the
                      magnitude of the hyperfine splittings compared to the
                      rotational-energy splittings plays a crucial role in the
                      spin-rotational dynamics after the laser pulse. Moreover, we
                      point out that the impact of the quadrupole coupling on the
                      rotational dynamics decreases when highly excited rotational
                      states dominate the dynamics.},
      cin          = {FS-CFEL-CMI / UNI/CUI / UNI/EXP},
      cid          = {I:(DE-H253)FS-CFEL-CMI-20220405 /
                      $I:(DE-H253)UNI_CUI-20121230$ /
                      $I:(DE-H253)UNI_EXP-20120731$},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631) / DFG project G:(GEPRIS)255652344 - SPP 1840:
                      Quantum Dynamics in Tailored Intense Fields (QUTIF)
                      (255652344) / DFG project G:(GEPRIS)194651731 - EXC 1074:
                      Hamburger Zentrum für ultraschnelle Beobachtung (CUI):
                      Struktur, Dynamik und Kontrolle von Materie auf atomarer
                      Skala (194651731) / AIM, DFG project G:(GEPRIS)390715994 -
                      EXC 2056: CUI: Advanced Imaging of Matter (390715994)},
      pid          = {G:(DE-HGF)POF4-631 / G:(GEPRIS)255652344 /
                      G:(GEPRIS)194651731 / G:(GEPRIS)390715994},
      experiment   = {EXP:(DE-MLZ)NOSPEC-20140101},
      typ          = {PUB:(DE-HGF)25},
      eprint       = {2408.01125},
      howpublished = {arXiv:2408.01125},
      archivePrefix = {arXiv},
      SLACcitation = {$\%\%CITATION$ = $arXiv:2408.01125;\%\%$},
      doi          = {10.3204/PUBDB-2024-01328},
      url          = {https://bib-pubdb1.desy.de/record/605154},
}