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@ARTICLE{Colaizzi:602233,
      author       = {Colaizzi, Lorenzo and Riabchuk, Sergei and Maansson, Erik
                      and Saraswathula, Krishna and Wanie, Vincent and Trabattoni,
                      Andrea and Gonzalez Vazquez, Jesus and Martin, Fernando and
                      Calegari, Francesca},
      title        = {{F}ew-femtosecond time-resolved study of the {UV}-induced
                      dissociative dynamics of iodomethane},
      journal      = {Nature Communications},
      volume       = {15},
      number       = {1},
      issn         = {2041-1723},
      address      = {[London]},
      publisher    = {Nature Publishing Group UK},
      reportid     = {PUBDB-2024-00541},
      pages        = {9196},
      year         = {2024},
      note         = {PIF-2021-03},
      abstract     = {We present a combined experimental and theoretical
                      investigation of the dissociative dynamics of iodomethane
                      following ultraviolet (UV) photoexcitation. Wedo so by using
                      a UV pump – near-infrared (NIR) probe scheme with an
                      unprecedented time resolution. The short duration of the UV
                      pulse (4.2 fs) allows the ultrafast dynamics to be
                      investigated in the absence of any external field, from well
                      before any significant vibrational displacement occurs until
                      dissociation has taken place. The experimental results are
                      used to benchmark semi-classical wave packet trajectory
                      calculations. In agreement with the experiment, the model
                      accurately identifies the main dissociation channels and
                      further reveals a clear signature of the conical
                      intersection in the time-dependent yield of the iodine ion.
                      Further, we demonstrate that the UV-induced breakage of the
                      C-I bond can be prevented when the molecule is ionized by
                      the probe pulse within 5 fs after UV light excitation,
                      showcasing an ultrafast stabilization scheme against
                      dissociation.},
      cin          = {FS-ATTO},
      ddc          = {500},
      cid          = {I:(DE-H253)FS-ATTO-20170403},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631) / DFG project G:(GEPRIS)390715994 - EXC 2056:
                      CUI: Advanced Imaging of Matter (390715994) / DFG project
                      G:(GEPRIS)194651731 - EXC 1074: Hamburger Zentrum für
                      ultraschnelle Beobachtung (CUI): Struktur, Dynamik und
                      Kontrolle von Materie auf atomarer Skala (194651731) / DFG
                      project G:(GEPRIS)170620586 - SFB 925: Licht-induzierte
                      Dynamik und Kontrolle korrelierter Quantensysteme
                      (170620586) / SoftMeter - Multi-messenger soft-field
                      spectroscopy of molecular electronics at interfaces
                      (101076500)},
      pid          = {G:(DE-HGF)POF4-631 / G:(GEPRIS)390715994 /
                      G:(GEPRIS)194651731 / G:(GEPRIS)170620586 /
                      G:(EU-Grant)101076500},
      experiment   = {EXP:(DE-MLZ)NOSPEC-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:39455555},
      UT           = {WOS:001342240600025},
      doi          = {10.1038/s41467-024-53183-8},
      url          = {https://bib-pubdb1.desy.de/record/602233},
}