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| Home > Publications database > Multifunctional Cellulose Nanofibrils–GdF$_3$ Nanoparticles Hybrid Gel and Its Potential Uses for Drug Delivery and Magnetic Resonance Imaging > print |
| Home > Publications database > Multifunctional Cellulose Nanofibrils–GdF$_3$ Nanoparticles Hybrid Gel and Its Potential Uses for Drug Delivery and Magnetic Resonance Imaging > print |
| 001 | 602025 | ||
| 005 | 20250715173435.0 | ||
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| 100 | 1 | _ | |a Jiang, Xuehe |0 P:(DE-H253)PIP1086595 |b 0 |
| 245 | _ | _ | |a Multifunctional Cellulose Nanofibrils–GdF$_3$ Nanoparticles Hybrid Gel and Its Potential Uses for Drug Delivery and Magnetic Resonance Imaging |
| 260 | _ | _ | |a Washington, DC |c 2023 |b ACS Publications |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a A multifunctional hybrid gel based on cellulose nanofibrils (CNFs) was developed by grafting on its surface stearyl acrylate (PSA) and gadolinium(III) fluoride nanoparticles (GdF$_3$ NPs) via Cu$^{0}$-mediated surface-initiated radical polymerization (SET-LRP) while encapsulating antimicrobial peptides in it. GdF$_3$ NPs were first surface-modified with 11-phosphonoundecyl acrylate (PDA) to participate in the SET-LRP and cross-linked the grafted polymer-modified CNF. Several characterizations of the hybrid material (GdF$_3$–PSA-CNF) were carried out, such as Fourier transform infrared (FTIR) spectroscopy, thermogravimetric analysis (TGA), rheology, and microscopic analyses. The grafted PSA and cross-linked GdF$_3$ NPs created sophisticated networks in the CNF-based gel, presenting outstanding rheological properties and promising three-dimensional (3D) printability of this hybrid material (GdF$_3$–PSA-CNF). The nanostructures of GdF$_3$ NPs and their incorporated CNF species were characterized via small-angle X-ray scattering (SAXS). In addition, due to the unique intrinsic property of the GdF$_3$ nanoparticles, properties for magnetic resonance imaging (MRI) of GdF$_3$–PSA-CNF were investigated, showing the potential application as a contrast agent. Finally, the encapsulation of the antimicrobial peptides added another function to the hybrid material, evaluated by an antimicrobial test against methicillin-resistant Staphylococcus aureus (MRSA) in vitro. |
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| 700 | 1 | _ | |a Mietner, J. Benedikt |b 1 |
| 700 | 1 | _ | |a Raveendran, Dhanya |0 P:(DE-H253)PIP1108989 |b 2 |
| 700 | 1 | _ | |a Ovchinnikov, Kirill V. |b 3 |
| 700 | 1 | _ | |a Sochor, Benedikt |0 P:(DE-H253)PIP1096609 |b 4 |
| 700 | 1 | _ | |a Mueller, Susanne |0 P:(DE-H253)PIP1098802 |b 5 |
| 700 | 1 | _ | |a Boehm-Sturm, Philipp |b 6 |
| 700 | 1 | _ | |a Lerouge, Frédéric |0 0000-0003-2909-527X |b 7 |
| 700 | 1 | _ | |a Chaput, Frédéric |0 0000-0002-5315-8675 |b 8 |
| 700 | 1 | _ | |a Gurikov, Pavel |b 9 |
| 700 | 1 | _ | |a Roth, Stephan V. |0 P:(DE-H253)PIP1003299 |b 10 |
| 700 | 1 | _ | |a Navarro, Julien R.G. |0 P:(DE-H253)PIP1107361 |b 11 |e Corresponding author |
| 773 | _ | _ | |a 10.1021/acsanm.3c04272 |g Vol. 6, no. 22, p. 21182 - 21193 |0 PERI:(DE-600)2916552-0 |n 22 |p 21182 - 21193 |t ACS applied nano materials |v 6 |y 2023 |x 2574-0970 |
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