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000602025 1001_ $$0P:(DE-H253)PIP1086595$$aJiang, Xuehe$$b0
000602025 245__ $$aMultifunctional Cellulose Nanofibrils–GdF$_3$ Nanoparticles Hybrid Gel and Its Potential Uses for Drug Delivery and Magnetic Resonance Imaging
000602025 260__ $$aWashington, DC$$bACS Publications$$c2023
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000602025 520__ $$aA multifunctional hybrid gel based on cellulose nanofibrils (CNFs) was developed by grafting on its surface stearyl acrylate (PSA) and gadolinium(III) fluoride nanoparticles (GdF$_3$ NPs) via Cu$^{0}$-mediated surface-initiated radical polymerization (SET-LRP) while encapsulating antimicrobial peptides in it. GdF$_3$ NPs were first surface-modified with 11-phosphonoundecyl acrylate (PDA) to participate in the SET-LRP and cross-linked the grafted polymer-modified CNF. Several characterizations of the hybrid material (GdF$_3$–PSA-CNF) were carried out, such as Fourier transform infrared (FTIR) spectroscopy, thermogravimetric analysis (TGA), rheology, and microscopic analyses. The grafted PSA and cross-linked GdF$_3$ NPs created sophisticated networks in the CNF-based gel, presenting outstanding rheological properties and promising three-dimensional (3D) printability of this hybrid material (GdF$_3$–PSA-CNF). The nanostructures of GdF$_3$ NPs and their incorporated CNF species were characterized via small-angle X-ray scattering (SAXS). In addition, due to the unique intrinsic property of the GdF$_3$ nanoparticles, properties for magnetic resonance imaging (MRI) of GdF$_3$–PSA-CNF were investigated, showing the potential application as a contrast agent. Finally, the encapsulation of the antimicrobial peptides added another function to the hybrid material, evaluated by an antimicrobial test against methicillin-resistant Staphylococcus aureus (MRSA) in vitro.
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000602025 7001_ $$aMietner, J. Benedikt$$b1
000602025 7001_ $$0P:(DE-H253)PIP1108989$$aRaveendran, Dhanya$$b2
000602025 7001_ $$aOvchinnikov, Kirill V.$$b3
000602025 7001_ $$0P:(DE-H253)PIP1096609$$aSochor, Benedikt$$b4
000602025 7001_ $$0P:(DE-H253)PIP1098802$$aMueller, Susanne$$b5
000602025 7001_ $$aBoehm-Sturm, Philipp$$b6
000602025 7001_ $$00000-0003-2909-527X$$aLerouge, Frédéric$$b7
000602025 7001_ $$00000-0002-5315-8675$$aChaput, Frédéric$$b8
000602025 7001_ $$aGurikov, Pavel$$b9
000602025 7001_ $$0P:(DE-H253)PIP1003299$$aRoth, Stephan V.$$b10
000602025 7001_ $$0P:(DE-H253)PIP1107361$$aNavarro, Julien R.G.$$b11$$eCorresponding author
000602025 773__ $$0PERI:(DE-600)2916552-0$$a10.1021/acsanm.3c04272$$gVol. 6, no. 22, p. 21182 - 21193$$n22$$p21182 - 21193$$tACS applied nano materials$$v6$$x2574-0970$$y2023
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