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@ARTICLE{Spahr:599925,
author = {Spahr, Dominik and Bayarjargal, Lkhamsuren and Haussühl,
Eiken and Luchitskaia, Rita and Friedrich, Alexandra and
Milman, Victor and Fedotenko, Timofey and Winkler, Björn},
title = {{T}wisted [{C}$_2${O}$_5$]$^{2−}$-groups in
{B}a[{C}$_2${O}$_5$] pyrocarbonate},
journal = {Chemical communications},
volume = {59},
number = {80},
issn = {0022-4936},
address = {Cambridge},
publisher = {Soc.},
reportid = {PUBDB-2023-07614},
pages = {11951 - 11954},
year = {2023},
note = {Waiting for fulltext},
abstract = {The inorganic pyrocarbonate salt Ba[C$_2$O$_5$] contains
twisted pyrocarbonate anions ([C$_2$O$_5$]$^{2−}$), an
atomic arrangement previously not observed in other
pyrocarbonates. This unexpected additional structural degree
of freedom points towards an enlarged chemical variability
in this novel group of compounds. Ba[C$_2$O$_5$] was
synthesized in a laser-heated diamond anvil cell at 30(2)
GPa by heating a mixture of Ba[CO$_3$] + CO$_2$ to ≈
1500(200) K. Its crystal structure was solved from single
crystal synchrotron X-ray diffraction data and confirmed by
density functional theory-based calculations. The two planar
[CO$_3$]$^{2−}$-groups of the [C$_2$O$_5$]$^{2−}$-anion
are strongly twisted around the bridging oxygen atom.
Ba[C$_2$O$_5$] has been observed in the pressure range of
5–30 GPa, where its symmetry is $P6/m$ with $Z=$12.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P02.2-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {37747265},
UT = {WOS:001072818800001},
doi = {10.1039/D3CC03324D},
url = {https://bib-pubdb1.desy.de/record/599925},
}