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@ARTICLE{Srensen:599109,
author = {Sørensen, Michael Korning and Gertsen, Anders Skovbo and
Fornari, Rocco Peter and Zhou, Binbin and Zhang, Xiaotong
and Jepsen, Peter Uhd and Stanzani, Edoardo and Yun, Shinhee
and Fernández Castro, Marcial and Schwartzkopf, Matthias
and Koutsioubas, Alexandros and de Silva, Piotr and
Espindola-Rodriguez, Moises and Kuhn, Luise Theil and
Andreasen, Jens Wenzel},
title = {{M}anipulating {O}rganic {S}emiconductor {M}orphology with
{V}isible {L}ight},
journal = {Advanced functional materials},
volume = {33},
number = {10},
issn = {1616-301X},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2023-07166},
pages = {2212835},
year = {2023},
abstract = {A method is presented to manipulate the final morphology of
roll-to-roll slot-die coated poly(3-hexylthiophene) (P3HT)
by optically exciting the p-type polymer in solution while
coating. These results provide a comprehensive picture of
the entire knowledge chain, from demonstrating how to apply
the authors’ method to a fundamental understanding of the
changes in morphology and physical properties induced by
exciting P3HT while coating. By combining results from
density functional theory and molecular dynamics simulations
with a variety of X-ray experiments, absorption
spectroscopy, and THz spectroscopy, the relationship between
morphology and physical properties of the thin film is
demonstrated. Specifically, in P3HT films excited with light
during deposition, changes in crystallinity and texture with
more face-on orientation and increased out-of-plane charge
mobility are observed.},
cin = {DOOR ; HAS-User / FS-PETRA-D},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PETRA-D-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P03-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000915534700001},
doi = {10.1002/adfm.202212835},
url = {https://bib-pubdb1.desy.de/record/599109},
}