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000599109 1001_ $$00000-0002-7031-2072$$aSørensen, Michael Korning$$b0
000599109 245__ $$aManipulating Organic Semiconductor Morphology with Visible Light
000599109 260__ $$aWeinheim$$bWiley-VCH$$c2023
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000599109 520__ $$aA method is presented to manipulate the final morphology of roll-to-roll slot-die coated poly(3-hexylthiophene) (P3HT) by optically exciting the p-type polymer in solution while coating. These results provide a comprehensive picture of the entire knowledge chain, from demonstrating how to apply the authors’ method to a fundamental understanding of the changes in morphology and physical properties induced by exciting P3HT while coating. By combining results from density functional theory and molecular dynamics simulations with a variety of X-ray experiments, absorption spectroscopy, and THz spectroscopy, the relationship between morphology and physical properties of the thin film is demonstrated. Specifically, in P3HT films excited with light during deposition, changes in crystallinity and texture with more face-on orientation and increased out-of-plane charge mobility are observed.
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000599109 7001_ $$0P:(DE-H253)PIP1085937$$aGertsen, Anders Skovbo$$b1
000599109 7001_ $$00000-0002-3792-8262$$aFornari, Rocco Peter$$b2
000599109 7001_ $$0P:(DE-H253)PIP1105938$$aZhou, Binbin$$b3
000599109 7001_ $$aZhang, Xiaotong$$b4
000599109 7001_ $$00000-0003-3915-1167$$aJepsen, Peter Uhd$$b5
000599109 7001_ $$0P:(DE-H253)PIP1096792$$aStanzani, Edoardo$$b6
000599109 7001_ $$0P:(DE-H253)PIP1100390$$aYun, Shinhee$$b7
000599109 7001_ $$00000-0003-3294-2994$$aFernández Castro, Marcial$$b8
000599109 7001_ $$0P:(DE-H253)PIP1010504$$aSchwartzkopf, Matthias$$b9
000599109 7001_ $$aKoutsioubas, Alexandros$$b10
000599109 7001_ $$ade Silva, Piotr$$b11
000599109 7001_ $$0P:(DE-H253)PIP1087956$$aEspindola-Rodriguez, Moises$$b12
000599109 7001_ $$0P:(DE-H253)PIP1087912$$aKuhn, Luise Theil$$b13
000599109 7001_ $$0P:(DE-H253)PIP1007357$$aAndreasen, Jens Wenzel$$b14$$eCorresponding author
000599109 773__ $$0PERI:(DE-600)2039420-2$$a10.1002/adfm.202212835$$gVol. 33, no. 10, p. 2212835$$n10$$p2212835$$tAdvanced functional materials$$v33$$x1616-301X$$y2023
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