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@ARTICLE{Chukova:597223,
author = {Chukova, Oksana and Borkovska, Lyudmyla and Khomenkova,
Larysa and Ponomaryov, Semyon and Androulidaki, Maria and
Stratakis, Emmanuel},
title = {{E}ffects of thermal treatment on the complex structure of
luminescence emission of {L}i-doped {Z}n{O} screen-printed
films},
journal = {Frontiers in physics},
volume = {11},
issn = {2296-424X},
address = {Lausanne},
publisher = {Frontiers Media},
reportid = {PUBDB-2023-06497},
pages = {1305114},
year = {2023},
abstract = {The ZnO–Li films were synthesized and investigated in an
attempt to explore and develop RE-free phosphor materials
capable of emitting intense visible light in a wide spectral
range. The effects of both heterovalent doping with lithium
and high-temperature annealing on the optical properties of
ZnO films were studied. The films were deposited on the
Al2O3 substrate using the screen-printing method and
annealed at 800–1,000°C in air for 0.5–3 h. Both doping
and annealing result in the transformation of the shape of
reflectance spectra in the range of 300–400 nm and the
shift of absorption edge to the long-wavelength region. At
the same time, the bandgap value estimated taking into
account the exciton peak position and its binding energy is
independent of Li-doping. The feature at 300–400 nm and
the shift of absorption edge are ascribed to the appearance
of the absorption band that excited the yellow
photoluminescence band. The photoluminescence spectra of
undoped and Li-doped films show the emission bands in the
ultraviolet and visible spectral ranges. The ultraviolet
emission is due to ZnO exciton recombination. The visible
emission band comprises several components peaked at 430,
482, 540, 575, and 640 nm. Their relative intensities depend
on Li-doping, annealing temperature, and annealing duration.
The 430- and 482-nm luminescence bands were observed in
Li-doped films only. Their excitation spectra show the peak
located at 330–340 nm, indicating that the energy
significantly exceeds the ZnO bandgap energy. Consequently,
the 430- and 482-nm luminescence bands are attributed to an
additional crystal phase formed under annealing. Other
components of visible emission bands are ascribed to the
defect-related emission of ZnO. The possible nature of these
bands is further discussed. Li-doping and annealing at
intermediate temperatures result in blue emission and an
enhancement of other visible bands, which makes ZnO–Li
films a perspective material in photonic applications.},
cin = {FS-PETRA-S},
ddc = {530},
cid = {I:(DE-H253)FS-PETRA-S-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
MSCA4Ukraine - MSCA4Ukraine (101101923) / NEP - Nanoscience
Foundries and Fine Analysis - Europe|PILOT (101007417)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(EU-Grant)101101923 / G:(EU-Grant)101007417},
experiment = {EXP:(DE-H253)P-P66-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001135606400001},
doi = {10.3389/fphy.2023.1305114},
url = {https://bib-pubdb1.desy.de/record/597223},
}