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@ARTICLE{Seyffertitz:596463,
      author       = {Seyffertitz, Malina and Stock, Sebastian and Rauscher, Max
                      Valentin and Prehal, Christian and Haas, Sylvio and Porcar,
                      Lionel and Paris, Oskar},
      title        = {{A}re {SAXS} and {SANS} suitable to extract information on
                      the role of water for electric-double-layer formation at the
                      carbon–aqueous-electrolyte interface?},
      journal      = {Faraday discussions},
      volume       = {249},
      issn         = {1359-6640},
      address      = {Cambridge [u.a.]},
      publisher    = {Soc.},
      reportid     = {PUBDB-2023-06157},
      pages        = {363 - 380},
      year         = {2023},
      abstract     = {This study reports on the applicability of X-ray
                      transmission (XRT), small- and wide-angle X-ray scattering
                      (SAXS/WAXS) and small-angle neutron scattering (SANS) for
                      investigating fundamental processes taking place in the
                      working electrode of an electric double-layer capacitor with
                      1 M RbBr aqueous electrolyte at different applied
                      potentials. XRT and incoherent neutron scattering are
                      employed to determine global ion- and water-concentration
                      changes and associated charge-balancing mechanisms. We
                      showcase the suitability of SAXS and SANS, respectively, to
                      get complementary information on local ion and solvent
                      rearrangement in nanoconfinement, but also underscore the
                      limitations of simple qualitative models, asking for more
                      quantitative descriptions of water–water and ion–water
                      interactions via detailed atomistic modelling approaches.},
      cin          = {DOOR ; HAS-User / FS-PET-D},
      ddc          = {540},
      cid          = {I:(DE-H253)HAS-User-20120731 /
                      I:(DE-H253)FS-PET-D-20190712},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3) /
                      FS-Proposal: I-20230206 EC (I-20230206-EC)},
      pid          = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3 /
                      G:(DE-H253)I-20230206-EC},
      experiment   = {EXP:(DE-H253)P-P62-20221101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {37795935},
      UT           = {WOS:001075804100001},
      doi          = {10.1039/D3FD00124E},
      url          = {https://bib-pubdb1.desy.de/record/596463},
}