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000588611 1001_ $$0P:(DE-H253)PIP1080965$$aYang, Zichen$$b0
000588611 245__ $$aResonant inelastic x-ray scattering from electronic excitations in $α$ − RuCl$_3$ nanolayers
000588611 260__ $$aWoodbury, NY$$bInst.$$c2023
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000588611 520__ $$aWe present Ru L$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of spin-orbit and $d−d$ excitations in exfoliated nanolayers of the Kitaev spin-liquid candidate RuCl$_3$. Whereas the spin-orbit excitations are independent of thickness, we observe a pronounced redshift and broadening of the $d−d$ excitations in layers with thicknesses below ∼7 nm. Aided by model calculations, we attribute these effects to distortions of the RuCl$_6$ octahedra near the surface. Our study paves the way towards RIXS investigations of electronic excitations in various other two-dimensional materials and heterostructures.  
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000588611 7001_ $$aWang, Lichen$$b1
000588611 7001_ $$00000-0002-7753-7637$$aZhao, Dong$$b2
000588611 7001_ $$00000-0002-0100-499X$$aLuo, Mingdi$$b3
000588611 7001_ $$00000-0002-4554-5042$$aLaha, Sourav$$b4
000588611 7001_ $$aGüth, Achim$$b5
000588611 7001_ $$aTaniguchi, Takashi$$b6
000588611 7001_ $$00000-0003-3701-8119$$aWatanabe, Kenji$$b7
000588611 7001_ $$00000-0002-3094-303X$$aLotsch, Bettina V.$$b8
000588611 7001_ $$0P:(DE-H253)PIP1020315$$aSmet, Jurgen H.$$b9
000588611 7001_ $$0P:(DE-H253)PIP1027117$$aMinola, Matteo$$b10
000588611 7001_ $$0P:(DE-H253)PIP1029079$$aGretarsson, Hlynur$$b11$$udesy
000588611 7001_ $$0P:(DE-H253)PIP1010052$$aKeimer, Bernhard$$b12$$eCorresponding author
000588611 773__ $$0PERI:(DE-600)2844160-6$$a10.1103/PhysRevB.108.L041406$$gVol. 108, no. 4, p. L041406$$n4$$pL041406$$tPhysical review / B$$v108$$x2469-9950$$y2023
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