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000588174 1001_ $$0P:(DE-H253)PIP1017464$$aHoffmann, Alexander$$b0
000588174 245__ $$aCatching an Entatic State-A Pair of Copper Complexes
000588174 260__ $$aWeinheim$$bWiley-VCH$$c2014
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000588174 520__ $$aThe structures of two types of guanidine–quinoline copper complexes have been investigated by single-crystal X-ray crystallography, K-edge X-ray absorption spectroscopy (XAS), resonance Raman and UV/Vis spectroscopy, cyclic voltammetry, and density functional theory (DFT). Independent of the oxidation state, the two structures, which are virtually identical for solids and complexes in solution, resemble each other strongly and are connected by a reversible electron transfer at 0.33 V. By resonant excitation of the two entatic copper complexes, the transition state of the electron transfer is accessible through vibrational modes, which are coupled to metal–ligand charge transfer (MLCT) and ligand–metal charge transfer (LMCT) states.
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000588174 7001_ $$aBinder, Stephan$$b1
000588174 7001_ $$0P:(DE-H253)PIP1020854$$aJesser, Anton$$b2
000588174 7001_ $$aHaase, Roxana$$b3
000588174 7001_ $$aFlörke, Ulrich$$b4
000588174 7001_ $$0P:(DE-H253)PIP1015176$$aGnida, Manuel$$b5
000588174 7001_ $$0P:(DE-H253)PIP1010984$$aSalomone Stagni, Marco$$b6
000588174 7001_ $$0P:(DE-H253)PIP1001970$$aMeyer-Klaucke, Wolfram$$b7$$udesy
000588174 7001_ $$0P:(DE-H253)PIP1018557$$aLebsanft, Benjamin$$b8
000588174 7001_ $$aGrünig, Lara Elena$$b9
000588174 7001_ $$aSchneider, Simon$$b10
000588174 7001_ $$aHashemi, Maryam$$b11
000588174 7001_ $$aGoos, Arne$$b12
000588174 7001_ $$0P:(DE-H253)PIP1020892$$aWetzel, Alina$$b13
000588174 7001_ $$aRübhausen, Michael$$b14
000588174 7001_ $$0P:(DE-H253)PIP1017463$$aHerres-Pawlis, Sonja$$b15$$eCorresponding author
000588174 773__ $$0PERI:(DE-600)2011836-3$$a10.1002/anie.201306061$$gVol. 53, no. 1, p. 299 - 304$$n1$$p299 - 304$$tAngewandte Chemie / International edition$$v53$$x1433-7851$$y2014
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