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@ARTICLE{VanCraen:586016,
author = {Van Craen, David and Kalarikkal, Malavika G. and Holstein,
Julian},
title = {{A} {C}harge-{N}eutral {S}elf-{A}ssembled {L}$_2${Z}n$_2$
{H}elicate as {B}ench-{S}table {R}eceptor for {A}nion
{R}ecognition at {N}anomolar {C}oncentration},
journal = {Journal of the American Chemical Society},
volume = {144},
number = {39},
issn = {0002-7863},
address = {Washington, DC},
publisher = {ACS Publications},
reportid = {PUBDB-2023-03743},
pages = {18135 - 18143},
year = {2022},
note = {Waiting for fulltext},
abstract = {The field of anion recognition chemistry is dominated by
two fundamental approaches to design receptors. One relies
on the formation of covalent bonds resulting in organic and
often neutral host species, while the other one utilizes
metal-driven self-assembly for the formation of charged
receptors with well-defined nanocavities. Yet, the
combination of their individual advantages in the form of
charge-neutral metal-assembled bench-stable anion receptors
is severely lacking. Herein, we present a fluorescent and
uncharged double-stranded hydroxyquinoline-based zinc(II)
helicate with the ability to bind environmentally relevant
dicarboxylate anions with high fidelity in dimethyl
sulfoxide (DMSO) at nanomolar concentrations. These dianions
are pinned between zinc(II) centers with binding constants
up to 145 000 000 M$^{–1}$. The presented
investigation exemplifies a pathway to bridge the two design
approaches and combine their strength in one structural
motif as an efficient anion receptor.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20210921
(I-20210921)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20210921},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {36137546},
UT = {WOS:000861632500001},
doi = {10.1021/jacs.2c08579},
url = {https://bib-pubdb1.desy.de/record/586016},
}