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@ARTICLE{Colombo:578452,
author = {Colombo, Alessandro and Dold, Simon and Kolb, Patrice and
Bernhardt, Nils and Behrens, Patrick and Correa Magdalena,
Jonathan and Düsterer, Stefan and Erk, Benjamin and Hecht,
Linos and Heilrath, Andrea and Irsig, Robert and Iwe, Norman
and Jordan, Jakob and Kruse, Bjoern and Langbehn, Bruno and
Manschwetus, Bastian and Martinez, Franklin and
Meiwes-Broer, Karl-Heinz and Oldenburg, Kevin and Passow,
Christopher and Peltz, Christian and Sauppe, Mario and Seel,
Fabian and Tanyag, Rico Mayro and Treusch, Rolf and Ulmer,
Anatoli and Walz, Saida and Fennel, Thomas and Barke, Ingo
and Moeller, Thomas and Von Issendorff, Bernd and Rupp,
Daniela},
title = {{T}hree-dimensional femtosecond snapshots of isolated
faceted nanostructures},
journal = {Science advances},
volume = {9},
number = {8},
issn = {2375-2548},
address = {Washington, DC [u.a.]},
publisher = {Assoc.},
reportid = {PUBDB-2023-00948},
pages = {eade5839},
year = {2023},
abstract = {The structure and dynamics of isolated nanosamples in free
flight can be directly visualized via single-shot coherent
diffractive imaging using the intense and short pulses of
x-ray free-electron lasers. Wide-angle scattering images
encode three-dimensional (3D) morphological information of
the samples, but its retrieval remains a challenge. Up to
now, effective 3D morphology reconstructions from single
shots were only achieved via fitting with highly constrained
models, requiring a priori knowledge about possible
geometries. Here, we present a much more generic imaging
approach. Relying on a model that allows for any sample
morphology described by a convex polyhedron, we reconstruct
wide-angle diffraction patterns from individual silver
nanoparticles. In addition to known structural motives with
high symmetries, we retrieve imperfect shapes and
agglomerates that were not previously accessible. Our
results open unexplored routes toward true 3D structure
determination of single nanoparticles and, ultimately, 3D
movies of ultrafast nanoscale dynamics.},
cin = {DOOR ; HAS-User / FS-FLASH-O / FS-DS / FS-FLASH-D / FS-LA /
$XFEL_E2_SQS$},
ddc = {500},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-FLASH-O-20160930 / I:(DE-H253)FS-DS-20120731 /
I:(DE-H253)FS-FLASH-D-20160930 / I:(DE-H253)FS-LA-20130416 /
$I:(DE-H253)XFEL_E2_SQS-20210408$},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G2 - FLASH (DESY) (POF4-6G2) / FS-Proposal:
F-20170541 (F-20170541)},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G2 /
G:(DE-H253)F-20170541},
experiment = {EXP:(DE-H253)F-BL1-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {36812315},
UT = {WOS:000949019100018},
doi = {10.1126/sciadv.ade5839},
url = {https://bib-pubdb1.desy.de/record/578452},
}