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000490786 1001_ $$0P:(DE-H253)PIP1090108$$aSingh, Himanshi$$b0
000490786 245__ $$aChiral control of gas‐phase molecules using microwave pulses
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000490786 520__ $$aMicrowave  three-wave  mixing  has  emerged  as  a  novel approach  for studying  chiral  molecules  in  the  gas phase.This technique employs resonant microwave pulses and is a non-linear and coherent approach. It serves as a robust method to differentiate between the enantiomers of chiral molecules and to determine the enantiomeric excess, even in complex chiral mixtures. Besides such analytical applications, the use of tailored microwave pulses allows us to control and manipulate chirality at the molecular level. Here, an overview  of  some  recent  developments  in  the area  of microwave three-wave  mixing and  its  extension  to  enantiomer-selective population transfer is provided. The latterisan important step towards enantiomer separation–in energy and finally in space. In the last section,  we  present  new  experimental  results on  how  to  improve enantiomer-selective population transfer to achieve an enantiomeric excess of about 40%in the rotational level of interest using microwave pulses alone.
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000490786 7001_ $$0P:(DE-H253)PIP1032339$$aBerggoetz, Freya Elsbeth Lieselotte$$b1
000490786 7001_ $$0P:(DE-H253)PIP1092107$$aSun, Wenhao$$b2$$eCorresponding author
000490786 7001_ $$0P:(DE-H253)PIP1013514$$aSchnell, Melanie$$b3$$eCorresponding author
000490786 773__ $$0PERI:(DE-600)2011836-3$$a10.1002/anie.202219045$$gVol. 62, no. 27, p. e202219045$$n27$$pe202219045$$tAngewandte Chemie / International edition$$v62$$x1433-7851$$y2023
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