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000490197 1001_ $$0P:(DE-H253)PIP1096981$$aCardoch, Sebastian$$b0$$eCorresponding author
000490197 245__ $$aDecreasing ultrafast X-ray pulse durations with saturable absorption and resonant transitions
000490197 260__ $$aWoodbury, NY$$bInst.$$c2023
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000490197 520__ $$aSaturable absorption is a nonlinear effect where a material’s ability to absorb light is frustrated due to a high influx of photons and the creation of electron vacancies. Experimentally induced saturable absorption in copper revealed a reduction in the temporal duration of transmitted X-ray laser pulses, but a detailed account of changes in opacity and emergence of resonances is still missing. In this computational work, we employ non-local thermodynamic equilibrium plasma simulations to study the interaction of femtosecond X-rays and copper. Following the onset of frustrated absorption, we find that a K–M resonant transition occurring at highly charged states turns copper opaque again. The changes in absorption generate a transient transparent window responsible for the shortened transmission signal. We also propose using fluorescence induced by the incident beam as an alternative source to achieve shorter X-ray pulses. Intense femtosecond X-rays are valuable to probe the structure and dynamics of biological samples or to reach extreme states of matter. Shortened pulses could be relevant for emerging imaging techniques.
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000490197 7001_ $$0P:(DE-H253)PIP1082226$$aTrost, Fabian$$b1
000490197 7001_ $$0P:(DE-H253)PIP1085046$$aScott, Howard$$b2
000490197 7001_ $$0P:(DE-H253)PIP1006324$$aChapman, Henry N.$$b3
000490197 7001_ $$0P:(DE-H253)PIP1011740$$aCaleman, Carl$$b4
000490197 7001_ $$0P:(DE-H253)PIP1008264$$aTimneanu, Nicusor$$b5$$eCorresponding author
000490197 773__ $$0PERI:(DE-600)2844562-4$$a10.1103/PhysRevE.107.015205$$gVol. 107, no. 1, p. 015205$$n1$$p015205$$tPhysical review / E$$v107$$x2470-0045$$y2023
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