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024 7 _ |a arXiv:2210.13162
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024 7 _ |a 10.1080/21663831.2023.2210606
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088 _ _ |a arXiv:2210.13162
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100 1 _ |a Lojewski, Tobias
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245 _ _ |a The interplay of local electron correlations and ultrafast spin dynamics in fcc Ni
260 _ _ |a London [u.a.]
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520 _ _ |a The complex electronic structure of metallic ferromagnets is determined by a balance betweenexchange interaction, electron hopping leading to band formation, and local Coulomb repulsion.By combining high energy and temporal resolution in femtosecond time-resolvedX-ray absorp-tion spectroscopy withab initiotime-dependent density functional theory we analyze the electronicstructure in fcc Ni on the time scale of these interactions in a pump-probe experiment. We distin-guish transient broadening and energy shifts in the absorption spectra, which we demonstrate to becaptured by electron repopulation respectively correlation-induced modifications of the electronicstructure, requiring to take the local Coulomb interaction into account.
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773 _ _ |a 10.1080/21663831.2023.2210606
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