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@ARTICLE{Graanaes:485207,
      author       = {Graanaes, Elin and Schröder, Ulrike A. and Arman, Mohammad
                      A. and Andersen, Mie and Gerber, Timm and Schulte, Karina
                      and Andersen, Jesper N. and Michely, Thomas and Hammer,
                      Bjørk and Knudsen, Jan},
      title        = {{W}ater {C}hemistry beneath {G}raphene: {C}ondensation of a
                      {D}ense {OH}–{H}$_2${O} {P}hase under {G}raphene},
      journal      = {The journal of physical chemistry / C},
      volume       = {126},
      number       = {9},
      issn         = {1932-7447},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {PUBDB-2022-06594},
      pages        = {4347 - 4354},
      year         = {2022},
      abstract     = {Room temperature oxygen hydrogenation below graphene flakes
                      supported by Ir(111) is investigated through a combination
                      of X-ray photoelectron spectroscopy, scanning tunneling
                      microscopy, and density functional theory calculations using
                      an evolutionary search algorithm. We demonstrate how the
                      graphene cover and its doping level can be used to trap and
                      characterize dense mixed O–OH–H$_2$O phases that
                      otherwise would not exist. Our study of these
                      graphene-stabilized phases and their response to oxygen or
                      hydrogen exposure reveals that additional oxygen can be
                      dissolved into them at room temperature creating mixed
                      O–OH–H$_2$O phases with an increased areal coverage
                      underneath graphene. In contrast, additional hydrogen
                      exposure converts the mixed O–OH–H$_2$O phases back to
                      pure OH–H$_2$O with a reduced areal coverage underneath
                      graphene.},
      cin          = {FS-NL},
      ddc          = {530},
      cid          = {I:(DE-H253)FS-NL-20120731},
      pnm          = {632 - Materials – Quantum, Complex and Functional
                      Materials (POF4-632)},
      pid          = {G:(DE-HGF)POF4-632},
      experiment   = {EXP:(DE-MLZ)External-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {35299819},
      UT           = {WOS:000772201900010},
      doi          = {10.1021/acs.jpcc.1c10289},
      url          = {https://bib-pubdb1.desy.de/record/485207},
}