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@ARTICLE{McManus:484476,
      author       = {McManus, Joseph W. and Walmsley, Tiffany and Nagaya,
                      Kiyonobu and Harries, James R. and Kumagai, Yoshiaki and
                      Iwayama, Hiroshi and Ashfold, Michael N. R. and Britton,
                      Mathew and Bucksbaum, Philip H. and Downes-Ward, Briony and
                      Driver, Taran and Heathcote, David and Hockett, Paul and
                      Howard, Andrew J. and Kukk, Edwin and Lee, Jason Wai Lung
                      and Liu, Yusong and Milesevic, Dennis and Minns, Russell S.
                      and Niozu, Akinobu and Niskanen, Johannes and Orr-Ewing,
                      Andrew J. and Owada, Shigeki and Rolles, Daniel and
                      Robertson, Patrick A. and Rudenko, Artem and Ueda, Kiyoshi
                      and Unwin, James and Vallance, Claire and Burt, Michael and
                      Brouard, Mark and Forbes, Ruaridh and Allum, Felix},
      title        = {{D}isentangling sequential and concerted fragmentations of
                      molecular polycations with covariant native frame analysis},
      journal      = {Physical chemistry, chemical physics},
      volume       = {24},
      number       = {37},
      issn         = {1463-9076},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {PUBDB-2022-06289},
      pages        = {22699 - 22709},
      year         = {2022},
      abstract     = {We present results from an experimental ion imaging study
                      into the fragmentation dynamics of 1-iodopropane and
                      2-iodopropane following interaction with extreme ultraviolet
                      intense femtosecond laser pulses with a photon energy of 95
                      eV. Using covariance imaging analysis, a range of observed
                      fragmentation pathways of the resulting polycations can be
                      isolated and interrogated in detail at relatively high ion
                      count rates (∼12 ions shot$^{−1}$). By incorporating the
                      recently developed native frames analysis approach into the
                      three-dimensional covariance imaging procedure,
                      contributions from three-body concerted and sequential
                      fragmentation mechanisms can be isolated. The angular
                      distribution of the fragment ions is much more complex than
                      in previously reported studies for triatomic polycations,
                      and differs substantially between the two isomeric species.
                      With support of simple simulations of the dissociation
                      channels of interest, detailed physical insights into the
                      fragmentation dynamics are obtained, including how the
                      initial dissociation step in a sequential mechanism
                      influences rovibrational dynamics in the metastable
                      intermediate ion and how signatures of this nuclear motion
                      manifest in the measured signals.},
      cin          = {FS-SMP},
      ddc          = {540},
      cid          = {I:(DE-H253)FS-SMP-20171124},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631)},
      pid          = {G:(DE-HGF)POF4-631},
      experiment   = {EXP:(DE-MLZ)External-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:36106844},
      UT           = {WOS:000854649200001},
      doi          = {10.1039/D2CP03029B},
      url          = {https://bib-pubdb1.desy.de/record/484476},
}