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000484476 1001_ $$aMcManus, Joseph W.$$b0
000484476 245__ $$aDisentangling sequential and concerted fragmentations of molecular polycations with covariant native frame analysis
000484476 260__ $$aCambridge$$bRSC Publ.$$c2022
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000484476 520__ $$aWe present results from an experimental ion imaging study into the fragmentation dynamics of 1-iodopropane and 2-iodopropane following interaction with extreme ultraviolet intense femtosecond laser pulses with a photon energy of 95 eV. Using covariance imaging analysis, a range of observed fragmentation pathways of the resulting polycations can be isolated and interrogated in detail at relatively high ion count rates (∼12 ions shot$^{−1}$). By incorporating the recently developed native frames analysis approach into the three-dimensional covariance imaging procedure, contributions from three-body concerted and sequential fragmentation mechanisms can be isolated. The angular distribution of the fragment ions is much more complex than in previously reported studies for triatomic polycations, and differs substantially between the two isomeric species. With support of simple simulations of the dissociation channels of interest, detailed physical insights into the fragmentation dynamics are obtained, including how the initial dissociation step in a sequential mechanism influences rovibrational dynamics in the metastable intermediate ion and how signatures of this nuclear motion manifest in the measured signals.
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000484476 7001_ $$aWalmsley, Tiffany$$b1
000484476 7001_ $$aNagaya, Kiyonobu$$b2
000484476 7001_ $$aHarries, James R.$$b3
000484476 7001_ $$aKumagai, Yoshiaki$$b4
000484476 7001_ $$aIwayama, Hiroshi$$b5
000484476 7001_ $$aAshfold, Michael N. R.$$b6
000484476 7001_ $$aBritton, Mathew$$b7
000484476 7001_ $$aBucksbaum, Philip H.$$b8
000484476 7001_ $$aDownes-Ward, Briony$$b9
000484476 7001_ $$aDriver, Taran$$b10
000484476 7001_ $$aHeathcote, David$$b11
000484476 7001_ $$aHockett, Paul$$b12
000484476 7001_ $$aHoward, Andrew J.$$b13
000484476 7001_ $$aKukk, Edwin$$b14
000484476 7001_ $$0P:(DE-H253)PIP1027857$$aLee, Jason Wai Lung$$b15
000484476 7001_ $$aLiu, Yusong$$b16
000484476 7001_ $$aMilesevic, Dennis$$b17
000484476 7001_ $$aMinns, Russell S.$$b18
000484476 7001_ $$00000-0002-7292-5630$$aNiozu, Akinobu$$b19
000484476 7001_ $$aNiskanen, Johannes$$b20
000484476 7001_ $$00000-0001-5551-9609$$aOrr-Ewing, Andrew J.$$b21
000484476 7001_ $$aOwada, Shigeki$$b22
000484476 7001_ $$0P:(DE-H253)PIP1007320$$aRolles, Daniel$$b23
000484476 7001_ $$00000-0003-0935-3331$$aRobertson, Patrick A.$$b24
000484476 7001_ $$aRudenko, Artem$$b25
000484476 7001_ $$aUeda, Kiyoshi$$b26
000484476 7001_ $$aUnwin, James$$b27
000484476 7001_ $$aVallance, Claire$$b28
000484476 7001_ $$aBurt, Michael$$b29
000484476 7001_ $$aBrouard, Mark$$b30
000484476 7001_ $$aForbes, Ruaridh$$b31
000484476 7001_ $$0P:(DE-HGF)0$$aAllum, Felix$$b32$$eCorresponding author
000484476 773__ $$0PERI:(DE-600)1476244-4$$a10.1039/D2CP03029B$$gVol. 24, no. 37, p. 22699 - 22709$$n37$$p22699 - 22709$$tPhysical chemistry, chemical physics$$v24$$x1463-9076$$y2022
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