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000481433 1001_ $$0P:(DE-H253)PIP1092439$$aHoeing, Dominik$$b0
000481433 245__ $$aTime-resolved single-particle x-ray scattering reveals electron-density gradients as coherent plasmonic-nanoparticle-oscillation source
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000481433 520__ $$aDynamics of optically excited plasmonic nanoparticles are presently understood as a series of scattering events involving the initiation of nanoparticle breathing oscillations. According to established models, these are caused by statistical heat transfer from thermalized electrons to the lattice. An additional contribution by hot-electron pressure accounts for phase mismatches between theory and experimental observations. However, direct experimental studies resolving the breathing-oscillation excitation are still missing. We used optical transient-absorption spectroscopy and time-resolved single-particle X-ray diffractive imaging to access the electron system and lattice. The time-resolved single-particle imaging data provided structural information directly on the onset of the breathing oscillation and confirmed the need for an additional excitation mechanism for thermal expansion. We developed a new model that reproduces all of our experimental observations. We identified optically induced electron density gradients as the initial driving source.
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000481433 7001_ $$0P:(DE-HGF)0$$aSelig, Malte$$b16
000481433 7001_ $$0P:(DE-HGF)0$$aKnorr, Andreas$$b17$$eCorresponding author
000481433 7001_ $$0P:(DE-H253)PIP1023449$$aAyyer, Kartik$$b18$$eCorresponding author
000481433 7001_ $$0P:(DE-H253)PIP1012175$$aKüpper, Jochen$$b19$$eCorresponding author
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000481433 7870_ $$0PUBDB-2024-01158$$aHoeing, Dominik et.al.$$d2023$$iIsParent$$rarXiv:2303.04513$$tTime-Resolved Single-Particle X-ray Scattering Reveals Electron-Density Gradients As Coherent Plasmonic-Nanoparticle-Oscillation Source
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