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100 1 _ |a Jacobse, Leon
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245 _ _ |a A combined rotating disk electrode - surface x-ray diffraction setup for surface structure characterization in electrocatalysis
260 _ _ |a [S.l.]
|c 2022
|b American Institute of Physics
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500 _ _ |a The following funding cannot be found in the database: We acknowledge financial support by the German Federal Ministry of Education and Research (BMBF projects 05K2016-HEXCHEM and 05K19WE1-CIXenergy). The authors acknowledge additional support by the Bavarian Ministry of Economic Affairs, Regional Development and Energy and the Deutsche Forschungsgemeinschaft (DFG) via the Collaborative Research Centre SFB 1452 (Catalysis at Liquid Interfaces , project 431791331), the Research Unit FOR 1878 (Functional Molecular Structures on Complex Oxide Surfaces, project 214951840) and further projects (431733372, 453560721)
520 _ _ |a Characterizing electrode surface structures under operando conditions is essential for fully understanding structure-activity relationships in electrocatalysis. Here, we combine in a single experiment, high-energy surface x-ray diffraction as characterizing technique with a rotating disk electrode to provide steady state kinetics under electrocatalytic conditions. Using Pt(111) and Pt(100) model electrodes, we show that full crystal truncation measurements are readily possible up to rotation rates of 1200 RPM. Furthermore, we discuss possibilities for both potentiostatic as well as potentiodynamic measurements, demonstrating the versatility of this technique. These different modes of operation, combined with the relatively simple experimental setup, make the combined rotating disk electrode - surface x-ray diffraction experiment a powerful technique for studying surface structures under operando electrocatalytic conditions.
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