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@ARTICLE{Degerman:477120,
author = {Degerman, David and Shipilin, Mikhail and Lömker, Patrick
and Goodwin, Christopher M. and Gericke, Sabrina M. and
Hejral, Uta and Gladh, Jörgen and Wang, Hsin-Yi and
Schlueter, Christoph and Nilsson, Anders and Amann, Peter},
title = {{O}perando {O}bservation of {O}xygenated {I}ntermediates
during {CO} {H}ydrogenation on {R}h {S}ingle {C}rystals},
journal = {Journal of the American Chemical Society},
volume = {144},
number = {16},
issn = {0002-7863},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {PUBDB-2022-01916},
pages = {7038 - 7042},
year = {2022},
abstract = {The CO hydrogenation reaction over the Rh(111) and (211)
surfaces has been investigated operando by X-ray
photoelectron spectroscopy at a pressure of 150 mbar.
Observations of the resting state of the catalyst give
mechanistic insight into the selectivity of Rh for
generating ethanol from CO hydrogenation. This study shows
that the Rh(111) surface does not dissociate all CO
molecules before hydrogenation of the O and C atoms, which
allows methoxy and other both oxygenated and hydrogenated
species to be visible in the photoelectron spectra.},
cin = {DOOR ; HAS-User / FS-PET-S},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PET-S-20190712},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G3 - PETRA III (DESY) (POF4-6G3) /
FS-Proposal: I-20191434 EC (I-20191434-EC) / SWEDEN-DESY -
SWEDEN-DESY Collaboration $(2020_Join2-SWEDEN-DESY)$},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G3 /
G:(DE-H253)I-20191434-EC /
$G:(DE-HGF)2020_Join2-SWEDEN-DESY$},
experiment = {EXP:(DE-H253)P-P22-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:35394273},
UT = {WOS:000799141600003},
doi = {10.1021/jacs.2c00300},
url = {https://bib-pubdb1.desy.de/record/477120},
}