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| 005 | 20250715175501.0 | ||
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| 088 | _ | _ | |a arXiv:2012.04852 |2 arXiv |
| 100 | 1 | _ | |a Schwickert, David |0 P:(DE-H253)PIP1021241 |b 0 |
| 245 | _ | _ | |a Electronic Quantum Coherence in Glycine Molecules Probed with Ultrashort X-ray Pulses in Real Time |
| 260 | _ | _ | |a Washington, DC [u.a.] |c 2022 |b Assoc. |
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| 520 | _ | _ | |a Here, we use x-rays to create and probe quantum coherence in the photoionized amino acid glycine. The outgoing photoelectron leaves behind the cation in a coherent superposition of quantum mechanical eigenstates. Delayed x-ray pulses track the induced coherence through resonant x-ray absorption that induces Auger decay and by photoelectron emission from sequential double photoionization. Sinusoidal temporal modulation of the detected signal at early times (0-25 fs) is observed in both measurements. Advanced ab initio many-electron simulations allow us to explain the first 25 fs of the detected coherent quantum evolution in terms of the electronic coherence. In the kinematically complete x-ray absorption measurement we monitor its dynamics for a period of 175 fs and observe an evolving modulation that may implicate the coupling of electronic to vibronic coherence at longer time scales. Our experiment provides a direct support for the existence of long-lived electronic coherence in photoionized biomolecules. |
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| 773 | _ | _ | |a 10.1126/sciadv.abn6848 |g Vol. 8, no. 22, p. eabn6848 |0 PERI:(DE-600)2810933-8 |n 22 |p eabn6848 |t Science advances |v 8 |y 2022 |x 2375-2548 |
| 787 | 0 | _ | |a Schwickert, David et.al. |d 2020 |i IsParent |0 PUBDB-2022-02957 |r arXiv:2012.04852 |t Electronic Quantum Coherence in Glycine Molecules Probed with Ultrashort X-ray Pulses in Real Time |
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