Home > Publications database > Picosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules > print

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024 7 _ |a 10.1038/s41467-022-28951-z
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100 1 _ |a Mullins, Terry
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245 _ _ |a Picosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules
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520 _ _ |a Fixing molecules in space is a crucial step for the imaging of molecular structure and dynamics. Here, we demonstrate three-dimensional (3D) field-free alignment of the proto- typical asymmetric top molecule indole using elliptically polarized, shaped, off-resonant laser pulses. A truncated laser pulse is produced using a combination of extreme linear chirping and controlled phase and amplitude shaping using a spatial-light-modulator (SLM) based pulse shaper of a broadband laser pulse. The angular confinement is detected through velocity-map imaging of H$^+$ and C$^{2+}$ fragments resulting from strong-field ionization and Coulomb explosion of the aligned molecules by intense femtosecond laser pulses. The achieved three-dimensional alignment is characterized by comparing the result of ion- velocity-map measurements for different alignment directions and for different times during and after the alignment laser pulse to accurate computational results. The achieved strong three-dimensional field-free alignment of <$cos^{2}δ4$> 0:89 demonstrates the feasibility of both, strong three-dimensional alignment of generic complex molecules and its quantitative characterization.
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700 1 _ |a Karamatskos, Evangelos Thomas
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700 1 _ |a Wiese, Joss
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700 1 _ |a Onvlee, Jolijn
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700 1 _ |a Küpper, Jochen
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773 _ _ |a 10.1038/s41467-022-28951-z
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787 0 _ |a Mullins, Terry et.al.
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|t Picosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules
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