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000476130 245__ $$aPicosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules
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000476130 520__ $$aFixing molecules in space is a crucial step for the imaging of molecular structure and dynamics. Here, we demonstrate three-dimensional (3D) field-free alignment of the proto- typical asymmetric top molecule indole using elliptically polarized, shaped, off-resonant laser pulses. A truncated laser pulse is produced using a combination of extreme linear chirping and controlled phase and amplitude shaping using a spatial-light-modulator (SLM) based pulse shaper of a broadband laser pulse. The angular confinement is detected through velocity-map imaging of H$^+$ and C$^{2+}$ fragments resulting from strong-field ionization and Coulomb explosion of the aligned molecules by intense femtosecond laser pulses. The achieved three-dimensional alignment is characterized by comparing the result of ion- velocity-map measurements for different alignment directions and for different times during and after the alignment laser pulse to accurate computational results. The achieved strong three-dimensional field-free alignment of <$cos^{2}δ4$> 0:89 demonstrates the feasibility of both, strong three-dimensional alignment of generic complex molecules and its quantitative characterization.
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000476130 7001_ $$0P:(DE-H253)PIP1025827$$aKaramatskos, Evangelos Thomas$$b1
000476130 7001_ $$0P:(DE-H253)PIP1022847$$aWiese, Joss$$b2
000476130 7001_ $$0P:(DE-H253)PIP1032788$$aOnvlee, Jolijn$$b3
000476130 7001_ $$0P:(DE-H253)PIP1008275$$aRouzée, Arnaud$$b4
000476130 7001_ $$0P:(DE-H253)PIP1031546$$aYachmenev, Andrey$$b5$$udesy
000476130 7001_ $$0P:(DE-H253)PIP1013309$$aTrippel, Sebastian$$b6
000476130 7001_ $$0P:(DE-H253)PIP1012175$$aKüpper, Jochen$$b7$$eCorresponding author
000476130 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-022-28951-z$$gVol. 13, no. 1, p. 1431$$n1$$p1431$$tNature Communications$$v13$$x2041-1723$$y2022
000476130 7870_ $$0PUBDB-2024-01858$$aMullins, Terry et.al.$$d2022$$iIsParent$$rarXiv:2009.08157$$tPicosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules
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