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000475846 1001_ $$0P:(DE-HGF)0$$aDe Bastiani, M. De$$b0$$eCorresponding author
000475846 245__ $$aMonolithic perovskite/silicon tandems with >28% efficiency: role of silicon-surface texture on perovskite properties
000475846 260__ $$aWeinheim$$bWiley-VCH$$c2023
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000475846 520__ $$aTextured silicon wafers used in silicon solar cell manufacturing offer superior light trapping, which is a critical enabler for high-performance photovoltaics. A similar optical benefit can be obtained in monolithic perovskite/silicon tandem solar cells, enhancing the current output of the silicon bottom cell. Yet, such complex silicon surfaces may affect the structural and optoelectronic properties of the overlying perovskite films. Here, through extensive characterization based on optical and microstructural spectroscopy, it is found that the main effect of such substrate morphology lies in an altering of the photoluminescence response of the perovskite, which is associated with thickness variations of the perovskite, rather than lattice strain or compositional changes. With this understanding, the design of high-performance perovskite/silicon tandems is rationalized, yielding certified power conversion efficiencies of >28%.
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000475846 7001_ $$0P:(DE-HGF)0$$aJalmood, R.$$b1
000475846 7001_ $$0P:(DE-HGF)0$$aLiu, J.$$b2
000475846 7001_ $$0P:(DE-H253)PIP1031991$$aOssig, Christina Sonja$$b3$$udesy
000475846 7001_ $$0P:(DE-HGF)0$$aVlk, A.$$b4
000475846 7001_ $$0P:(DE-HGF)0$$aVegso, K.$$b5
000475846 7001_ $$0P:(DE-HGF)0$$aBabics, M.$$b6
000475846 7001_ $$0P:(DE-HGF)0$$aIsikgor, F. H.$$b7
000475846 7001_ $$0P:(DE-HGF)0$$aSelvin, A. S.$$b8
000475846 7001_ $$0P:(DE-HGF)0$$aAzmi, R.$$b9
000475846 7001_ $$0P:(DE-HGF)0$$aUgur, E.$$b10
000475846 7001_ $$0P:(DE-HGF)0$$aBanerjee, S.$$b11
000475846 7001_ $$0P:(DE-HGF)0$$aMirabelli, A. J.$$b12
000475846 7001_ $$0P:(DE-HGF)0$$aAydin, E.$$b13
000475846 7001_ $$0P:(DE-HGF)0$$aAllen, T. G.$$b14
000475846 7001_ $$0P:(DE-HGF)0$$aRehman, A. U.$$b15
000475846 7001_ $$0P:(DE-HGF)0$$aVan Kerschaver, E.$$b16
000475846 7001_ $$0P:(DE-HGF)0$$aSiffalovic, P.$$b17
000475846 7001_ $$0P:(DE-H253)PIP1081708$$aStückelberger, Michael$$b18$$udesy
000475846 7001_ $$0P:(DE-HGF)0$$aLedinsky, M.$$b19
000475846 7001_ $$0P:(DE-HGF)0$$aDe Wolf, S.$$b20
000475846 773__ $$0PERI:(DE-600)2039420-2$$a10.1002/adfm.202205557$$gp. 2205557 -$$n4$$p2205557$$tAdvanced functional materials$$v33$$x1616-301X$$y2023
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000475846 8564_ $$uhttps://bib-pubdb1.desy.de/record/475846/files/De%20Bastiani%20et%20al_advanced%20materials_manuscript.pdf$$yPublished on 2022-12-09. Available in OpenAccess from 2023-12-09.
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