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000475352 1001_ $$0P:(DE-H253)PIP1082049$$aPotorochin, Dmitrii$$b0$$eCorresponding author$$udesy
000475352 245__ $$aSurface functionalization of few-layer graphene on β -SiC(001) by Neutral Red dye
000475352 260__ $$aAmsterdam$$bElsevier$$c2022
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000475352 520__ $$aFew-layer graphene on -SiC(001) functionalized with phenazine dye Neutral Red by means of diazonium chemistry has been studied using X-ray photoelectron spectroscopy, near-edge X-ray absorption fine structure, photoemission electron microscopy, scanning tunneling microscopy, and density functional theory calculations. The experimental data reveal the formation of a composite phenazine dye/graphene structure with a large energy gap. The molecules in this structure can be oriented both parallel and perpendicular to the graphene surface. According to scanning tunneling spectroscopy and theoretical calculations, the density of electron states in different surface areas depends on the local short-range order and the molecules’ environment. On the other hand, the photoemission spectroscopy study shows that the bottom layers of the few-layer graphene remain intact, which inherently makes the synthesized layered composite a low-dimensional metal/semiconductor heterostructure. In addition, photoemission electron microscopy imaging shows a high homogeneity of the dye-modified graphene on a micrometer scale.
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000475352 7001_ $$0P:(DE-HGF)0$$aChaika, Alexander N.$$b1
000475352 7001_ $$0P:(DE-H253)PIP1015516$$aMolodtsova, Olga$$b2$$udesy
000475352 7001_ $$0P:(DE-H253)PIP1016125$$aAristov, Victor$$b3
000475352 7001_ $$0P:(DE-HGF)0$$aMarchenko, Dmitry E.$$b4
000475352 7001_ $$0P:(DE-HGF)0$$aSmirnov, Dmitry A.$$b5
000475352 7001_ $$0P:(DE-HGF)0$$aMakarova, Anna A.$$b6
000475352 7001_ $$0P:(DE-HGF)0$$aWalls, Brian$$b7
000475352 7001_ $$0P:(DE-HGF)0$$aZhussupbekov, Kuanysh$$b8
000475352 7001_ $$0P:(DE-HGF)0$$aWalshe, Killian$$b9
000475352 7001_ $$0P:(DE-HGF)0$$aShvets, Igor V.$$b10
000475352 7001_ $$0P:(DE-H253)PIP1016690$$aCiobanu, Anca Simona$$b11$$udesy
000475352 7001_ $$0P:(DE-HGF)0$$aRabchinskii, Maxim K.$$b12
000475352 7001_ $$0P:(DE-HGF)0$$aUlin, Nikolai V.$$b13
000475352 7001_ $$0P:(DE-HGF)0$$aBaidakova, Marina V.$$b14
000475352 7001_ $$0P:(DE-HGF)0$$aBrunkov, Pavel N.$$b15
000475352 7001_ $$0P:(DE-H253)PIP1007192$$aMolodtsov, Serguei$$b16
000475352 773__ $$0PERI:(DE-600)2002520-8$$a10.1016/j.apsusc.2022.152542$$gVol. 585, p. 152542 -$$p152542$$tApplied surface science$$v585$$x0169-4332$$y2022
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