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@ARTICLE{Garg:475232,
author = {Garg, Diksha and Lee, Jason Wai Lung and Tikhonov, Denis
and Chopra, Pragya and Steber, Amanda and Lemmens, Alexander
and Erk, Benjamin and Allum, Felix and Boll, Rebecca and
Cheng, Xuemei and Duesterer, Stefan and Gruet, Sebastien
Patrice and He, Lanhai and Heathcote, David and Johny, Melby
and Mohammad Kazemi, Mehdi and Koeckert, Hansjochen and
Lahl, Jan and Loru, Donatella and Maclot, Sylvain and Mason,
Robert and Mueller, Erland and Mullins, Terence and Olshin,
Pavel and Passow, Christopher and Peschel, Jasper and Ramm,
Daniel and Rompotis, Dimitrios and Trippel, Sebastian and
Wiese, Joss and Ziaee, Farzaneh and Bari, Sadia and Burt,
Michael and Küpper, Jochen and Rijs, Anouk and Rolles,
Daniel and Techert, Simone and Eng-Johnsson, Per and
Brouard, Mark and Vallance, Claire and Manschwetus, Bastian
and Schnell, Melanie},
title = {{F}ragmentation dynamics of fluorene explored using
ultrafast {XUV}-{V}is pump-probe spectroscopy},
journal = {Frontiers in physics},
volume = {10},
issn = {2296-424X},
address = {Lausanne},
publisher = {Frontiers Media},
reportid = {PUBDB-2022-01289},
pages = {880793},
year = {2022},
abstract = {We report on the use of extreme ultraviolet (XUV, 30.3 nm)
radiation from the Free-electron LASer in Hamburg (FLASH)
and visible (Vis, 405 nm) photons from an optical laser to
investigate the relaxation and fragmentation dynamics of
fluorene ions. The ultrashort laser pulses allow to resolve
the molecular processes occurring on the femtosecond
timescales. Fluorene is a prototypical small polycyclic
aromatic hydrocarbon (PAH). Through their infrared emission
signature, PAHs have been shown to be ubiquitous in the
universe, and they are assumed to play an important role in
the chemistry of the interstellar medium. Our experiments
track the ionization and dissociative ionization products of
fluorene through time-of-flight mass spectrometry and
velocity-map imaging. Multiple processes involved in the
formation of each of the fragment ions are disentangled
through analysis of the ion images. The relaxation lifetimes
of the excited fluorene monocation and dication obtained
through the fragment formation channels are reported to be
in the range of a few tens of femtoseconds to a few
picoseconds.},
cin = {FS-SMP / FS-SCS / FS-CFEL-CMI / UNI/CUI / UNI/EXP /
FS-FLASH-O},
ddc = {530},
cid = {I:(DE-H253)FS-SMP-20171124 / I:(DE-H253)FS-SCS-20131031 /
I:(DE-H253)FS-CFEL-CMI-20220405 /
$I:(DE-H253)UNI_CUI-20121230$ /
$I:(DE-H253)UNI_EXP-20120731$ /
I:(DE-H253)FS-FLASH-O-20160930},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / 6G2 - FLASH (DESY) (POF4-6G2) / FS-Proposal:
F-20170540 (F-20170540) / DFG project 390715994 - EXC 2056:
CUI: Advanced Imaging of Matter (390715994) / DFG project
194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle
Beobachtung (CUI): Struktur, Dynamik und Kontrolle von
Materie auf atomarer Skala (194651731) / HIRS-0018 -
Helmholtz-Lund International School - Intelligent
instrumentation for exploring matter at different time and
length scales (HELIOS) $(2020_HIRS-0018)$},
pid = {G:(DE-HGF)POF4-631 / G:(DE-HGF)POF4-6G2 /
G:(DE-H253)F-20170540 / G:(GEPRIS)390715994 /
G:(GEPRIS)194651731 / $G:(DE-HGF)2020_HIRS-0018$},
experiment = {EXP:(DE-H253)F-BL1-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000804771900001},
doi = {10.3389/fphy.2022.880793},
url = {https://bib-pubdb1.desy.de/record/475232},
}