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@ARTICLE{Hoppe:474968,
author = {Hoppe, Uwe and Schöps, A. and Hannon, Alex and Barz, A.
and Stachel, D.},
title = {{S}tructure of binary antimony phosphate glasses by
diffraction methods},
journal = {Journal of non-crystalline solids},
volume = {583},
issn = {0022-3093},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PUBDB-2022-01094},
pages = {121476 -},
year = {2022},
abstract = {Antimony phosphate glasses
(Sb$_2$O$_3$)x(P$_2$O$_5$)$_{1-x}$ with $x$ = 0.05 and 0.80
were measured by neutron and X-ray diffraction with high
real-space resolution. The P−O and O−O distance peaks of
the PO$_4$ tetrahedra were found with the expected
parameters. For the glass of $x$ = 0.80 the Sb−O and O−O
coordination numbers and distances suggest highly distorted
SbO$_3$ and SbO$_4$ environments according to strong
lone-pair effects of the Sb$^{3+}$. The fraction of SbO$_4$
has the right portion that all oxygens can form Sb−O−Sb
or Sb−O−P bridges. Significant numbers of secondary
Sb−O bonds (> 0.25 nm) are extracted. The first
diffraction peak at 13 nm$^{−1}$ is related to distances
between stacked layers of corner-connected oxygen triangles
as in the orthorhombic Sb$_2$O$_3$. For the glass of $x$ =
0.05 the medium-range order reminds that of vitreous
P$_2$O$_5$. Its SbO$_4$ units are formed with mean Sb−O
bonds of 0.210 nm.},
cin = {FS-DO / FS-US},
ddc = {670},
cid = {I:(DE-H253)FS-DO-20120731 / I:(DE-H253)FS-US-20120731},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631)},
pid = {G:(DE-HGF)POF4-631},
experiment = {EXP:(DE-H253)D-BW5-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000789673600004},
doi = {10.1016/j.jnoncrysol.2022.121476},
url = {https://bib-pubdb1.desy.de/record/474968},
}