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@ARTICLE{Robinson:473651,
author = {Robinson, Matthew S. and Niebuhr, Mario and Lever, Fabiano
and Mayer, Dennis and Metje, Jan and Gühr, Markus},
title = {{U}ltrafast {P}hoto-ion {P}robing of the {R}ing-{O}pening
{P}rocess in {T}rans-{S}tilbene {O}xide},
journal = {Chemistry - a European journal},
volume = {27},
number = {44},
issn = {0947-6539},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2022-00164},
pages = {11418 - 11427},
year = {2021},
abstract = {The ultrafast photo-induced ring opening of the oxirane
derivative trans-stilbene oxide has been studied through the
use of ultrafast UV/UV pump-probe spectroscopy by using
photo-ion detection. Single- and multiphoton probe paths and
final states were identified through comparisons between UV
power studies and synchrotron-based vacuum ultraviolet (VUV)
single-photon ionization studies. Three major time-dependent
features of the parent ion (sub-450 fs decay,
(1.5±0.2) ps, and >100 ps) were observed. These decays
are discussed in conjunction with the primary ring-opening
mechanism of stilbene oxide, which occurs through C−C
dissociation in the oxirane ring. The appearance of
fragments relating to the masses of dehydrogenated
diphenylmethane (167 amu) and dehydrogenated methylbenzene
(90 amu) were also investigated. The appearance of the
167 amu fragment could suggest an alternative ultrafast
ring-opening pathway via the dissociation of one of the
C−O bonds within the oxirane ring.},
cin = {FS-CFEL-CMI},
ddc = {540},
cid = {I:(DE-H253)FS-CFEL-CMI-20220405},
pnm = {633 - Life Sciences – Building Blocks of Life: Structure
and Function (POF4-633)},
pid = {G:(DE-HGF)POF4-633},
experiment = {EXP:(DE-MLZ)External-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:34037274},
UT = {WOS:000662737000001},
doi = {10.1002/chem.202101343},
url = {https://bib-pubdb1.desy.de/record/473651},
}