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@ARTICLE{Borzutzki:463159,
author = {Borzutzki, Kristina and Dong, Kang and Nair, Jijeesh Ravi
and Wolff, Beatrice and Hausen, Florian and Eichel,
Rüdiger-A. and Winter, Martin and Manke, Ingo and
Brunklaus, Gunther},
title = {{L}ithium deposition in single-ion conducting polymer
electrolytes},
journal = {Cell reports},
volume = {2},
number = {7},
issn = {2666-3864},
address = {[New York, NY]},
publisher = {Elsevier},
reportid = {PUBDB-2021-03660},
pages = {100496},
year = {2021},
abstract = {Lithium (Li)-metal is considered as promising anode
material for high-energy-density rechargeable batteries,
although its application is hampered by inhomogeneous Li
deposition and dendritic Li morphologies that could
eventually result in contact losses of bulk and deposited Li
as well as cell short circuits. Based on theoretical
investigations, recent works on polymer electrolytes
particularly focus on the design of single-ion conducting
electrolytes and improvement of bulk Li$^+$ transport
properties, including enhanced Li$^+$ transference numbers,
ionic conductivity, and mechanical stability, thereby
affording safer and potentially “dendrite-free” cycling
of Li-metal batteries. In the present work, it is revealed
that the spatial microstructures, localized chemistry, and
corresponding distributions of properties within the
electrolyte are also decisive for achieving superior cell
performances. Thus, targeted modification of the electrolyte
microstructures should be considered as further critical
design parameters for future electrolyte development and to
actually control Li deposition behavior and longevity of
Li-metal batteries.},
cin = {DOOR ; HAS-User / Hereon},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 / I:(DE-H253)Hereon-20210428},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P05-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000677677000006},
doi = {10.1016/j.xcrp.2021.100496},
url = {https://bib-pubdb1.desy.de/record/463159},
}