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024 7 _ |a 10.1038/s41467-021-26772-0
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100 1 _ |a Yang, Yudong
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245 _ _ |a Strong-field coherent control of isolated attosecond pulse generation
260 _ _ |a London
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520 _ _ |a Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: improved spectral tunability (allowing selectivity in addressing electronic transitions) and higher photon flux (permitting to measure low cross-section processes). New developments come through parametric waveform synthesis, which provides control over the shape of field transients, enabling the creation of highly-tunable isolated attosecond pulses via high-harmonic generation. Here we demonstrate that the first goal is fulfilled since central energy, spectral bandwidth/shape and temporal duration of isolated attosecond pulses can be controlled by shaping the laser waveform via two key parameters: the relative-phase between two halves of the multi-octave spanning spectrum, and the overall carrier-envelope phase. These results not only promise to expand the experimental possibilities in attosecond science, but also demonstrate coherent strong-field control of free-electron trajectories using tailored optical waveforms.
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536 _ _ |a DFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)
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700 1 _ |a Mainz, Roland E.
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700 1 _ |a Rossi, Giulio Maria
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700 1 _ |a Scheiba, Fabian
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700 1 _ |a Silva Toledo, Miguel Angel
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700 1 _ |a Keathley, Phillip D.
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700 1 _ |a Cirmi, Giovanni
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700 1 _ |a Kärtner, Franz
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773 _ _ |a 10.1038/s41467-021-26772-0
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