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024 | 7 | _ | |a 10.1038/s41467-021-25347-3 |2 doi |
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100 | 1 | _ | |a Pressacco, Federico |0 P:(DE-H253)PIP1027495 |b 0 |e Corresponding author |
245 | _ | _ | |a Subpicosecond metamagnetic phase transition in FeRh driven by non-equilibrium electron dynamics |
260 | _ | _ | |a [London] |c 2021 |b Nature Publishing Group UK |
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520 | _ | _ | |a Femtosecond light-induced phase transitions between different macroscopic orders provide the possibility to tune the functional properties of condensed matter on ultrafast timescales. In first-order phase transitions, transient non-equilibrium phases and inherent phase coexistence often preclude non-ambiguous detection of transition precursors and their temporal onset.Here, we present a study combining time-resolved photoelectron spectroscopy and ab-initio electron dynamics calculations elucidating the transient subpicosecond processes governing the photoinduced generation of ferromagnetic order in antiferromagnetic {F}e{R}h. The transient photoemission spectra are accounted for by assuming that not only the occupation of electronic states is modified during the photoexcitation process.Instead, the photo-generated non-thermal distribution of electrons modifies the electronic band structure. The ferromagnetic phase of FeRh, characterized by a minority band near the Fermi energy, is established $ 350 \pm 30$ fs after the laser excitation. Ab-initio calculations indicate that the phase transition is initiated by a photoinduced Rh-to-Fe charge transfer. |
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773 | _ | _ | |a 10.1038/s41467-021-25347-3 |0 PERI:(DE-600)2553671-0 |p 5088 |t Nature Communications |v 12 |y 2021 |x 2041-1723 |
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