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000459421 088__ $$2arXiv$$aarXiv:2105.00764
000459421 1001_ $$0P:(DE-HGF)0$$aSchouder, Constant Alexandre$$b0
000459421 245__ $$aLaser-induced Coulomb explosion imaging of $(C_6$$H_5$$Br)$$_2$ and $C_6$$H_5$$Br$-$I_2$ dimers in helium nanodroplets using the Timepix3
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000459421 520__ $$aWe have deduced the structure of the bromobenzene-$I_2$ heterodimer and the bromobenzene homodimer inside helium droplets using a combination of laser-induced alignment, Coulomb explosion imaging, and three-dimensional ion imaging. The complexes were fixed in a variety of orientations in the laboratory frame, then in each case multiply ionized by an intense laser pulse. A three dimensional ion imaging detector, including a Timepix3 detector allowed us to measure the correlations between velocity vectors of different fragments and, in conjunction with classical simulations, work backward to the initial structure of the complex prior to explosion. For the heterodimer, we find that the $I_2$ molecular axis intersects the phenyl ring of the bromobenzene approximately perpendicularly. The homodimer has a stacked parallel structure, with the two bromine atoms pointing in opposite directions. These results illustrate the ability of Coulomb explosion imaging to determine the structure of large complexes, and point the way toward real-time measurements of bimolecular reactions inside helium droplets.
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000459421 650_7 $$2Other$$aAtomic and Molecular Clusters (physics.atm-clus)
000459421 650_7 $$2Other$$aChemical Physics (physics.chem-ph)
000459421 650_7 $$2Other$$aOptics (physics.optics)
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000459421 7001_ $$0P:(DE-HGF)0$$aChatterley, Adam Simon$$b1
000459421 7001_ $$0P:(DE-H253)PIP1028301$$aJohny, Melby$$b2
000459421 7001_ $$0P:(DE-HGF)0$$aHübschmann, Flora$$b3
000459421 7001_ $$0P:(DE-H253)PIP1081972$$aAl-Refaie, Ahmed$$b4
000459421 7001_ $$0P:(DE-HGF)0$$aCalvo, Florent$$b5
000459421 7001_ $$0P:(DE-H253)PIP1012175$$aKüpper, Jochen$$b6
000459421 7001_ $$0P:(DE-H253)PIP1085121$$aStapelfeldt, Henrik$$b7$$eCorresponding author
000459421 770__ $$z0953-4075
000459421 773__ $$0PERI:(DE-600)1363381-8$$a10.1088/1361-6455/ac04c4$$gVol. 54, no. 18, p. 184001 -$$n18$$p184001$$tJournal of physics / B$$v54$$x0022-3700$$y2021
000459421 7870_ $$0PUBDB-2024-01850$$aSchouder, Constant et.al.$$d2021$$iIsParent$$rarXiv:2105.00764$$tLaser-induced Coulomb explosion imaging of $(C_6$$H_5$$Br)$$_2$ and $C_6$$H_5$$Br$-$I_2$ dimers in helium nanodroplets using the Timepix3 
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