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| 001 | 458619 | ||
| 005 | 20250724175446.0 | ||
| 024 | 7 | _ | |a 10.1002/anie.202103178 |2 doi |
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| 100 | 1 | _ | |a Peresypkina, Eugenia |0 P:(DE-H253)PIP1027099 |b 0 |
| 245 | _ | _ | |a Three‐Component Self‐Assembly Changes its Course: A Leap from Simple Polymers to 3D Networks of Spherical Host–Guest Assemblies |
| 260 | _ | _ | |a Weinheim |c 2021 |b Wiley-VCH |
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| 520 | _ | _ | |a One-pot self-assembly reactions of the polyphosphoruscomplex [Cp*Fe($\eta^5$-P$_5$)] (A), a coinage metal saltAgSbF$_6$, and flexible aliphatic dinitriles NC(CH$_2$)$_x$CN (x=1–10) yield 1D, 2D, and 3D coordination polymers. The sevenmemberedbackbone of the dinitrile was experimentally foundas the borderline for the self-assembly system furnishingproducts of different kinds. At x<7, various rather simplepolymers are exclusively formed possessing either 0D or 1DAg/A structural motifs connected by dinitrile spacers, while at x$\geq$+7, the self-assembly switches to unprecedented extraordinary3D networks of nano-sized host–guest assemblies(SbF$_6$)@[(A)$_9$Ag$_{11}$]$^{11+}$ (x=7) or (A)@[(A)$_{12}$Ag$_{12}$]$^{12+}$ (x=8–10) linked by dinitriles. The polycationic nodes represent thefirst superspheres based on A and silver and are host–guestable. All products are characterized by NMR spectroscopy,mass spectrometry, and single-crystal X-ray diffraction. Theassemblies [(A)$_{12}$Ag$_{12}$]$^{12+}$ were visualized by transmissionelectron microscopy. |
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| 700 | 1 | _ | |a Grill, Kevin |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Hiltl, Barbara |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Virovets, Alexandr |0 P:(DE-H253)PIP1026845 |b 3 |
| 700 | 1 | _ | |a Kremer, Werner |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Hilgert, Jan |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Tremel, Wolfgang |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Scheer, Manfred |0 P:(DE-H253)PIP1027085 |b 7 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/anie.202103178 |g Vol. 60, no. 21, p. 12132 - 12142 |0 PERI:(DE-600)2011836-3 |n 21 |p 12132 - 12142 |t Angewandte Chemie / International edition |v 60 |y 2021 |x 1521-3773 |
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