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@ARTICLE{Peresypkina:458619,
      author       = {Peresypkina, Eugenia and Grill, Kevin and Hiltl, Barbara
                      and Virovets, Alexandr and Kremer, Werner and Hilgert, Jan
                      and Tremel, Wolfgang and Scheer, Manfred},
      title        = {{T}hree‐{C}omponent {S}elf‐{A}ssembly {C}hanges its
                      {C}ourse: {A} {L}eap from {S}imple {P}olymers to 3{D}
                      {N}etworks of {S}pherical {H}ost–{G}uest {A}ssemblies},
      journal      = {Angewandte Chemie / International edition},
      volume       = {60},
      number       = {21},
      issn         = {1521-3773},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {PUBDB-2021-02272},
      pages        = {12132 - 12142},
      year         = {2021},
      abstract     = {One-pot self-assembly reactions of the
                      polyphosphoruscomplex [Cp*Fe($\eta^5$-P$_5$)] (A), a coinage
                      metal saltAgSbF$_6$, and flexible aliphatic dinitriles
                      NC(CH$_2$)$_x$CN (x=1–10) yield 1D, 2D, and 3D
                      coordination polymers. The sevenmemberedbackbone of the
                      dinitrile was experimentally foundas the borderline for the
                      self-assembly system furnishingproducts of different kinds.
                      At x<7, various rather simplepolymers are exclusively formed
                      possessing either 0D or 1DAg/A structural motifs connected
                      by dinitrile spacers, while at x$\geq$+7, the self-assembly
                      switches to unprecedented extraordinary3D networks of
                      nano-sized host–guest
                      assemblies(SbF$_6$)@[(A)$_9$Ag$_{11}$]$^{11+}$ (x=7) or
                      (A)@[(A)$_{12}$Ag$_{12}$]$^{12+}$ (x=8–10) linked by
                      dinitriles. The polycationic nodes represent thefirst
                      superspheres based on A and silver and are host–guestable.
                      All products are characterized by NMR spectroscopy,mass
                      spectrometry, and single-crystal X-ray diffraction.
                      Theassemblies [(A)$_{12}$Ag$_{12}$]$^{12+}$ were visualized
                      by transmissionelectron microscopy.},
      cin          = {DOOR ; HAS-User},
      ddc          = {540},
      cid          = {I:(DE-H253)HAS-User-20120731},
      pnm          = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20160654
                      (I-20160654) / FS-Proposal: I-20180967 (I-20180967)},
      pid          = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20160654 /
                      G:(DE-H253)I-20180967},
      experiment   = {EXP:(DE-H253)P-P11-20150101 / EXP:(DE-H253)P-P24-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:33686782},
      UT           = {WOS:000646323700001},
      doi          = {10.1002/anie.202103178},
      url          = {https://bib-pubdb1.desy.de/record/458619},
}