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@ARTICLE{Heinl:458618,
author = {Heinl, Claudia and Peresypkina, Eugenia and Balázs, Gábor
and Mädl, Eric and Virovets, Alexandr and Scheer, Manfred},
title = {{T}he {M}issing {P}arent {C}ompound
$[({C}_{5}{H}_{5}){F}e(η^{5}‐{P}_{5})]$: {S}ynthesis,
{C}haracterization, {C}oordination {B}ehavior and
{E}ncapsulation},
journal = {Chemistry - a European journal},
volume = {27},
number = {27},
issn = {1521-3765},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2021-02271},
pages = {7542 - 7548},
year = {2021},
abstract = {The so far missing parent compound of the large family of
pentaphosphaferrocenes
[(C$_{5}$H$_{5}$)Fe($η^{5}‐P_{5})]$ (1 b) was
synthesized by the thermolysis of [CpFe(CO)$_2$]$_2$ with
P$_4$ using the very high-boiling solvent
diisopropylbenzene. It was comprehensively characterized by,
inter alia, NMR spectroscopy, single crystal X-ray structure
analysis, cyclic voltammetry and DFT computations. Moreover,
its coordination behavior towards CuI halides was explored,
revealing the unprecedented 2D polymeric networks
[{CpFe($η^{5:1:1:1:1}$-P$_5$)}Cu$_2$(μ-X)$_2$]$_n$ (2 a:
X=Cl, 2 b: X=Br) and
[{CpFe($η^{5:1:1}$-P$_5$)}Cu(μ-I)]$_n$ (3) and even the
first cyclo-P5-containing 3D coordination polymer
[{CpFe($η^{5:1:1}$-P$_5$)}Cu(μ-I)]$_n$ (4). The sandwich
complex 1 b can also be incorporated in nano-sized
supramolecules based on [Cp*Fe($η^5 -P_5$)] (1 a) and CuX
(X=Cl, Br, I): [CpFe($η^5 -P_5$)]@[{Cp*Fe($η^5
-P_5$)}$_{12}$(CuX)$_{20-n}$] (5 a: X=Cl, n=2.4; 5 b:
X=Br, n=2.4; 5 c: X=I, n=0.95). Thereby, the formation of
the CuI-containing fullerene-like sphere 5 c is found for
the first time.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20160654
(I-20160654)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20160654},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:33543820},
UT = {WOS:000627477800001},
doi = {10.1002/chem.202100203},
url = {https://bib-pubdb1.desy.de/record/458618},
}