guest ::
| Home > Publications database > Correlation-driven sub-3 fs charge migration in ionised adenine > print |
| Home > Publications database > Correlation-driven sub-3 fs charge migration in ionised adenine > print |
| 001 | 456289 | ||
| 005 | 20240619210130.0 | ||
| 024 | 7 | _ | |a arXiv:2101.05753 |2 arXiv |
| 024 | 7 | _ | |a 10.3204/PUBDB-2021-01440 |2 datacite_doi |
| 037 | _ | _ | |a PUBDB-2021-01440 |
| 041 | _ | _ | |a English |
| 100 | 1 | _ | |a Mansson, Erik P. |0 P:(DE-H253)PIP1082891 |b 0 |
| 245 | _ | _ | |a Correlation-driven sub-3 fs charge migration in ionised adenine |
| 260 | _ | _ | |c 2021 |
| 336 | 7 | _ | |a Preprint |b preprint |m preprint |0 PUB:(DE-HGF)25 |s 1718800792_3801547 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a WORKING_PAPER |2 ORCID |
| 336 | 7 | _ | |a Electronic Article |0 28 |2 EndNote |
| 336 | 7 | _ | |a preprint |2 DRIVER |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a Output Types/Working Paper |2 DataCite |
| 520 | _ | _ | |a Sudden ionisation of a relatively large molecule can initiate a correlation-driven process dubbed charge migration, where the electron density distribution is expected to rapidly change. Capturing this few-femtosecond/attosecond charge redistribution represents the real-time observation of the electron correlation in the molecule. So far, there has been no experimental evidence of this process. Here we report on a time-resolved study of the correlation-driven charge migration process occurring in the bio-relevant molecule adenine after ionisation by a 15-35 eV attosecond pulse. We find that, the production of intact doubly charged adenine - via a shortly-delayed laser-induced second ionisation event - represents the signature of a charge inflation mechanism resulting from the many-body excitation. This conclusion is supported by first-principles time-dependent simulations. Our findings opens new important perspectives for the control of the molecular reactivity at the electronic timescale. |
| 536 | _ | _ | |a 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) |0 G:(DE-HGF)POF4-631 |c POF4-631 |f POF IV |x 0 |
| 536 | _ | _ | |a STARLIGHT - Steering attosecond electron dynamics in biomolecules with UV-XUV LIGHT pulses (637756) |0 G:(EU-Grant)637756 |c 637756 |f ERC-2014-STG |x 1 |
| 536 | _ | _ | |a HIRS-0018 - Helmholtz-Lund International School - Intelligent instrumentation for exploring matter at different time and length scales (HELIOS) (2020_HIRS-0018) |0 G:(DE-HGF)2020_HIRS-0018 |c 2020_HIRS-0018 |x 2 |
| 536 | _ | _ | |a DFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731) |0 G:(GEPRIS)194651731 |c 194651731 |x 3 |
| 536 | _ | _ | |a DFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994) |0 G:(GEPRIS)390715994 |c 390715994 |x 4 |
| 588 | _ | _ | |a Dataset connected to DataCite |
| 693 | _ | _ | |0 EXP:(DE-MLZ)NOSPEC-20140101 |5 EXP:(DE-MLZ)NOSPEC-20140101 |e No specific instrument |x 0 |
| 700 | 1 | _ | |a Latini, Simone |0 P:(DE-H253)PIP1033049 |b 1 |
| 700 | 1 | _ | |a Covito, Fabio |0 P:(DE-H253)PIP1027772 |b 2 |
| 700 | 1 | _ | |a Wanie, Vincent |0 P:(DE-H253)PIP1083947 |b 3 |
| 700 | 1 | _ | |a Galli, Mara |0 P:(DE-H253)PIP1083941 |b 4 |
| 700 | 1 | _ | |a Perfetto, Enrico |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Stefanucci, Gianluca |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Huebener, Hannes |0 P:(DE-H253)PIP1032009 |b 7 |
| 700 | 1 | _ | |a De Giovannini, Umberto |0 P:(DE-H253)PIP1081134 |b 8 |
| 700 | 1 | _ | |a Castrovilli, Mattea C. |0 P:(DE-H253)PIP1091874 |b 9 |
| 700 | 1 | _ | |a Trabattoni, Andrea |0 P:(DE-H253)PIP1028302 |b 10 |
| 700 | 1 | _ | |a Frassetto, Fabio |0 P:(DE-H253)PIP1011527 |b 11 |
| 700 | 1 | _ | |a Poletto, Luca |0 P:(DE-H253)PIP1011519 |b 12 |
| 700 | 1 | _ | |a Greenwood, Jason B. |0 P:(DE-HGF)0 |b 13 |
| 700 | 1 | _ | |a Legare, Francois |0 P:(DE-HGF)0 |b 14 |
| 700 | 1 | _ | |a Nisoli, Mauro |0 P:(DE-HGF)0 |b 15 |
| 700 | 1 | _ | |a Rubio, Angel |0 P:(DE-H253)PIP1023770 |b 16 |
| 700 | 1 | _ | |a Calegari, Francesca |0 P:(DE-H253)PIP1023238 |b 17 |e Corresponding author |
| 856 | 4 | _ | |u https://arxiv.org/abs/2101.05753 |
| 856 | 4 | _ | |u https://bib-pubdb1.desy.de/record/456289/files/fulltext%20%28copied%20from%20arXiv%29.pdf |y OpenAccess |
| 856 | 4 | _ | |u https://bib-pubdb1.desy.de/record/456289/files/fulltext%20%28copied%20from%20arXiv%29.pdf?subformat=pdfa |x pdfa |y OpenAccess |
| 909 | C | O | |o oai:bib-pubdb1.desy.de:456289 |p openaire |p open_access |p driver |p VDB |p ec_fundedresources |p dnbdelivery |
| 910 | 1 | _ | |a Deutsches Elektronen-Synchrotron |0 I:(DE-588b)2008985-5 |k DESY |b 0 |6 P:(DE-H253)PIP1082891 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 1 |6 P:(DE-H253)PIP1033049 |
| 910 | 1 | _ | |a Max-Planck-Gesellschaft zur Förderung der Wissenschaften |0 I:(DE-588b)2019024-4 |k MPG |b 1 |6 P:(DE-H253)PIP1033049 |
| 910 | 1 | _ | |a Max-Planck-Gesellschaft zur Förderung der Wissenschaften |0 I:(DE-588b)2019024-4 |k MPG |b 2 |6 P:(DE-H253)PIP1027772 |
| 910 | 1 | _ | |a Deutsches Elektronen-Synchrotron |0 I:(DE-588b)2008985-5 |k DESY |b 3 |6 P:(DE-H253)PIP1083947 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 3 |6 P:(DE-H253)PIP1083947 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 4 |6 P:(DE-H253)PIP1083941 |
| 910 | 1 | _ | |a External Institute |0 I:(DE-HGF)0 |k Extern |b 4 |6 P:(DE-H253)PIP1083941 |
| 910 | 1 | _ | |a Deutsches Elektronen-Synchrotron |0 I:(DE-588b)2008985-5 |k DESY |b 4 |6 P:(DE-H253)PIP1083941 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 7 |6 P:(DE-H253)PIP1032009 |
| 910 | 1 | _ | |a Max-Planck-Gesellschaft zur Förderung der Wissenschaften |0 I:(DE-588b)2019024-4 |k MPG |b 7 |6 P:(DE-H253)PIP1032009 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 8 |6 P:(DE-H253)PIP1081134 |
| 910 | 1 | _ | |a External Institute |0 I:(DE-HGF)0 |k Extern |b 9 |6 P:(DE-H253)PIP1091874 |
| 910 | 1 | _ | |a European XFEL |0 I:(DE-588)1043621512 |k XFEL.EU |b 9 |6 P:(DE-H253)PIP1091874 |
| 910 | 1 | _ | |a Deutsches Elektronen-Synchrotron |0 I:(DE-588b)2008985-5 |k DESY |b 10 |6 P:(DE-H253)PIP1028302 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 10 |6 P:(DE-H253)PIP1028302 |
| 910 | 1 | _ | |a External Institute |0 I:(DE-HGF)0 |k Extern |b 11 |6 P:(DE-H253)PIP1011527 |
| 910 | 1 | _ | |a External Institute |0 I:(DE-HGF)0 |k Extern |b 12 |6 P:(DE-H253)PIP1011519 |
| 910 | 1 | _ | |a Centre for Free-Electron Laser Science |0 I:(DE-H253)_CFEL-20120731 |k CFEL |b 16 |6 P:(DE-H253)PIP1023770 |
| 910 | 1 | _ | |a Max-Planck-Gesellschaft zur Förderung der Wissenschaften |0 I:(DE-588b)2019024-4 |k MPG |b 16 |6 P:(DE-H253)PIP1023770 |
| 910 | 1 | _ | |a Deutsches Elektronen-Synchrotron |0 I:(DE-588b)2008985-5 |k DESY |b 17 |6 P:(DE-H253)PIP1023238 |
| 913 | 1 | _ | |a DE-HGF |b Forschungsbereich Materie |l Von Materie zu Materialien und Leben |1 G:(DE-HGF)POF4-630 |0 G:(DE-HGF)POF4-631 |3 G:(DE-HGF)POF4 |2 G:(DE-HGF)POF4-600 |4 G:(DE-HGF)POF |v Matter – Dynamics, Mechanisms and Control |x 0 |
| 913 | 0 | _ | |a DE-HGF |b Forschungsbereich Materie |l Von Materie zu Materialien und Leben |1 G:(DE-HGF)POF3-620 |0 G:(DE-HGF)POF3-621 |3 G:(DE-HGF)POF3 |2 G:(DE-HGF)POF3-600 |4 G:(DE-HGF)POF |v In-house research on the structure, dynamics and function of matter |9 G:(DE-HGF)POF3-6211 |x 0 |
| 914 | 1 | _ | |y 2021 |
| 915 | _ | _ | |a OpenAccess |0 StatID:(DE-HGF)0510 |2 StatID |
| 915 | _ | _ | |a Creative Commons Attribution CC BY 4.0 |0 LIC:(DE-HGF)CCBY4 |2 HGFVOC |
| 915 | _ | _ | |a Published |0 StatID:(DE-HGF)0580 |2 StatID |
| 920 | 1 | _ | |0 I:(DE-H253)FS-ATTO-20170403 |k FS-ATTO |l Attosecond Science and Technology |x 0 |
| 920 | 1 | _ | |0 I:(DE-H253)CFEL-MPT-20160915 |k CFEL-MPT |l MPSD |x 1 |
| 980 | _ | _ | |a preprint |
| 980 | _ | _ | |a VDB |
| 980 | _ | _ | |a I:(DE-H253)FS-ATTO-20170403 |
| 980 | _ | _ | |a I:(DE-H253)CFEL-MPT-20160915 |
| 980 | _ | _ | |a UNRESTRICTED |
| 980 | 1 | _ | |a FullTexts |
| Library | Collection | CLSMajor | CLSMinor | Language | Author |
|---|