000456289 001__ 456289
000456289 005__ 20240619210130.0
000456289 0247_ $$2arXiv$$aarXiv:2101.05753
000456289 0247_ $$2datacite_doi$$a10.3204/PUBDB-2021-01440
000456289 037__ $$aPUBDB-2021-01440
000456289 041__ $$aEnglish
000456289 1001_ $$0P:(DE-H253)PIP1082891$$aMansson, Erik P.$$b0
000456289 245__ $$aCorrelation-driven sub-3 fs charge migration in ionised adenine
000456289 260__ $$c2021
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000456289 520__ $$aSudden ionisation of a relatively large molecule can initiate a correlation-driven process dubbed charge migration, where the electron density distribution is expected to rapidly change. Capturing this few-femtosecond/attosecond charge redistribution represents the real-time observation of the electron correlation in the molecule. So far, there has been no experimental evidence of this process. Here we report on a time-resolved study of the correlation-driven charge migration process occurring in the bio-relevant molecule adenine after ionisation by a 15-35 eV attosecond pulse. We find that, the production of intact doubly charged adenine - via a shortly-delayed laser-induced second ionisation event - represents the signature of a charge inflation mechanism resulting from the many-body excitation. This conclusion is supported by first-principles time-dependent simulations. Our findings opens new important perspectives for the control of the molecular reactivity at the electronic timescale.
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000456289 536__ $$0G:(EU-Grant)637756$$aSTARLIGHT - Steering attosecond electron dynamics in biomolecules with UV-XUV LIGHT pulses (637756)$$c637756$$fERC-2014-STG$$x1
000456289 536__ $$0G:(DE-HGF)2020_HIRS-0018$$aHIRS-0018 - Helmholtz-Lund International School - Intelligent instrumentation for exploring matter at different time and length scales (HELIOS) (2020_HIRS-0018)$$c2020_HIRS-0018$$x2
000456289 536__ $$0G:(GEPRIS)194651731$$aDFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)$$c194651731$$x3
000456289 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x4
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000456289 7001_ $$0P:(DE-H253)PIP1033049$$aLatini, Simone$$b1
000456289 7001_ $$0P:(DE-H253)PIP1027772$$aCovito, Fabio$$b2
000456289 7001_ $$0P:(DE-H253)PIP1083947$$aWanie, Vincent$$b3
000456289 7001_ $$0P:(DE-H253)PIP1083941$$aGalli, Mara$$b4
000456289 7001_ $$0P:(DE-HGF)0$$aPerfetto, Enrico$$b5
000456289 7001_ $$0P:(DE-HGF)0$$aStefanucci, Gianluca$$b6
000456289 7001_ $$0P:(DE-H253)PIP1032009$$aHuebener, Hannes$$b7
000456289 7001_ $$0P:(DE-H253)PIP1081134$$aDe Giovannini, Umberto$$b8
000456289 7001_ $$0P:(DE-H253)PIP1091874$$aCastrovilli, Mattea C.$$b9
000456289 7001_ $$0P:(DE-H253)PIP1028302$$aTrabattoni, Andrea$$b10
000456289 7001_ $$0P:(DE-H253)PIP1011527$$aFrassetto, Fabio$$b11
000456289 7001_ $$0P:(DE-H253)PIP1011519$$aPoletto, Luca$$b12
000456289 7001_ $$0P:(DE-HGF)0$$aGreenwood, Jason B.$$b13
000456289 7001_ $$0P:(DE-HGF)0$$aLegare, Francois$$b14
000456289 7001_ $$0P:(DE-HGF)0$$aNisoli, Mauro$$b15
000456289 7001_ $$0P:(DE-H253)PIP1023770$$aRubio, Angel$$b16
000456289 7001_ $$0P:(DE-H253)PIP1023238$$aCalegari, Francesca$$b17$$eCorresponding author
000456289 8564_ $$uhttps://arxiv.org/abs/2101.05753
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000456289 9141_ $$y2021
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