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@ARTICLE{Saribal:456183,
      author       = {Saribal, Cem and Owens, Alec and Yachmenev, Andrey and
                      Küpper, Jochen},
      title        = {{D}etecting handedness of spatially oriented molecules by
                      {C}oulomb explosion imaging},
      journal      = {The journal of chemical physics},
      volume       = {154},
      number       = {7},
      issn         = {1089-7690},
      address      = {Melville, NY},
      publisher    = {American Institute of Physics},
      reportid     = {PUBDB-2021-01390},
      pages        = {071101},
      year         = {2021},
      abstract     = {We present a new technique for detecting chirality in the
                      gas phase: Chiral molecules are spatially aligned in three
                      dimensions by a moderately strong elliptically polarized
                      laser field. The momentum distributions of the charged
                      fragments, produced by laser-induced Coulomb explosion, show
                      distinct three-dimensional orientation of the enantiomers
                      when the laser polarization ellipse is rotated by a
                      non-right angle with respect to the norm vector of the
                      detector plane. The resulting velocity-map-image asymmetry
                      is directly connected to the enantiomeric excess and to the
                      absolute handedness of molecules. We demonstrated our scheme
                      computationally for camphor (C10H16O), with its methyl
                      groups as marker fragments, using quantum-mechanical
                      simulations geared toward experimentally feasible
                      conditions. Computed sensitivity to enantiomeric excess is
                      comparable to other modern chiroptical approaches. The
                      present method can be readily optimized for any chiral
                      molecule with an anisotropic polarizability tensor by
                      adjusting the polarization state and intensity profile of
                      the laser field.},
      cin          = {FS-CFEL-1 / FS-CFEL-CMI / UNI/CUI / UNI/EXP},
      ddc          = {530},
      cid          = {I:(DE-H253)FS-CFEL-1-20120731 /
                      I:(DE-H253)FS-CFEL-CMI-20220405 /
                      $I:(DE-H253)UNI_CUI-20121230$ /
                      $I:(DE-H253)UNI_EXP-20120731$},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631) / DFG project 390715994 - EXC 2056: CUI: Advanced
                      Imaging of Matter (390715994) / DFG project 194651731 - EXC
                      1074: Hamburger Zentrum für ultraschnelle Beobachtung
                      (CUI): Struktur, Dynamik und Kontrolle von Materie auf
                      atomarer Skala (194651731) / DFG project 255652344 - SPP
                      1840: Quantum Dynamics in Tailored Intense Fields (QUTIF)
                      (255652344) / Ex-Net-0002-Phase2-3 - Advanced Imaging of
                      Matter: Structure, Dynamics and Control on the Atomic Scale
                      - AIM $(2018_Ex-Net-0002-Phase2-3)$},
      pid          = {G:(DE-HGF)POF4-631 / G:(GEPRIS)390715994 /
                      G:(GEPRIS)194651731 / G:(GEPRIS)255652344 /
                      $G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$},
      experiment   = {EXP:(DE-MLZ)NOSPEC-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:33607914},
      UT           = {WOS:000630521200001},
      doi          = {10.1063/5.0029792},
      url          = {https://bib-pubdb1.desy.de/record/456183},
}