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@ARTICLE{Li:455143,
      author       = {Li, Nian and Chen, Wei and Song, Lin and Guo, Renjun and
                      Scheel, Manuel A. and Yang, Dan and Körstgens, Volker and
                      Schwartzkopf, Matthias and Roth, Stephan V. and
                      Müller-Buschbaum, Peter},
      title        = {{I}n {S}itu {S}tudy of {O}rder {F}ormation in {M}esoporous
                      {T}itania {T}hin {F}ilms {T}emplated by a {D}iblock
                      {C}opolymer during {S}lot-{D}ie {P}rinting},
      journal      = {ACS applied materials $\&$ interfaces},
      volume       = {12},
      number       = {51},
      issn         = {1944-8252},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {PUBDB-2021-00958},
      pages        = {57627 - 57637},
      year         = {2020},
      note         = {Waiting for fulltext},
      abstract     = {Slot-die printing, a large-scale deposition technique, is
                      applied to fabricate mesoporous titania films. Printing is
                      interesting, for example, for scaling up solar cells where
                      titania films with an interconnected mesoporous network and
                      a large surface-to-volume ratio are desired as photoanodes.
                      A fundamental understanding of the structure evolution
                      during printing is of high significance in tailoring these
                      films. In this work, we provide important insights into the
                      self-assembly of the slot-die-printed
                      titania/polystyrene-block-poly(ethylene oxide) (PS-b-PEO)
                      micelles into ordered hybrid structures in real time via in
                      situ grazing-incidence small-angle X-ray scattering
                      (GISAXS). GISAXS allows for tracking both vertical and
                      lateral structure development of the film formation process.
                      In the hybrid film, a face-centered cubic (FCC) structure is
                      preferentially formed at the interfaces with air and with
                      the substrate, while a defect-rich mixed FCC and
                      body-centered cubic (BCC) structure forms in the bulk. After
                      calcination, the surface and inner morphologies of the
                      obtained nanostructured titania films are compared with the
                      spin-coated analogues. In the printed films, the initially
                      formed nanoscale structure of the hybrid film is preserved,
                      and the resulting mesoporous titania film shows a superior
                      order as compared with the spin-coated thin films which can
                      be beneficial for future applications.},
      cin          = {DOOR ; HAS-User / FS-PET-D},
      ddc          = {600},
      cid          = {I:(DE-H253)HAS-User-20120731 /
                      I:(DE-H253)FS-PET-D-20190712},
      pnm          = {6214 - Nanoscience and Materials for Information Technology
                      (POF3-621) / 6G3 - PETRA III (POF3-622) / SWEDEN-DESY -
                      SWEDEN-DESY Collaboration $(2020_Join2-SWEDEN-DESY)$ / DFG
                      project 390776260 - EXC 2089: e-conversion (390776260)},
      pid          = {G:(DE-HGF)POF3-6214 / G:(DE-HGF)POF3-6G3 /
                      $G:(DE-HGF)2020_Join2-SWEDEN-DESY$ / G:(GEPRIS)390776260},
      experiment   = {EXP:(DE-H253)P-P03-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:33295752},
      UT           = {WOS:000603397200095},
      doi          = {10.1021/acsami.0c18851},
      url          = {https://bib-pubdb1.desy.de/record/455143},
}